Laboratório Nacional de Ciência e Tecnologia do Bioetanol (CTBE), Centro Nacional de Pesquisa em Energia e Materiais (CNPEM), Campinas, São Paulo, Brasil.
PLoS One. 2013 Jul 29;8(7):e70014. doi: 10.1371/journal.pone.0070014. Print 2013.
Metagenomics has been widely employed for discovery of new enzymes and pathways to conversion of lignocellulosic biomass to fuels and chemicals. In this context, the present study reports the isolation, recombinant expression, biochemical and structural characterization of a novel endoxylanase family GH10 (SCXyl) identified from sugarcane soil metagenome. The recombinant SCXyl was highly active against xylan from beechwood and showed optimal enzyme activity at pH 6,0 and 45°C. The crystal structure was solved at 2.75 Å resolution, revealing the classical (β/α)8-barrel fold with a conserved active-site pocket and an inherent flexibility of the Trp281-Arg291 loop that can adopt distinct conformational states depending on substrate binding. The capillary electrophoresis analysis of degradation products evidenced that the enzyme displays unusual capacity to degrade small xylooligosaccharides, such as xylotriose, which is consistent to the hydrophobic contacts at the +1 subsite and low-binding energies of subsites that are distant from the site of hydrolysis. The main reaction products from xylan polymers and phosphoric acid-pretreated sugarcane bagasse (PASB) were xylooligosaccharides, but, after a longer incubation time, xylobiose and xylose were also formed. Moreover, the use of SCXyl as pre-treatment step of PASB, prior to the addition of commercial cellulolytic cocktail, significantly enhanced the saccharification process. All these characteristics demonstrate the advantageous application of this enzyme in several biotechnological processes in food and feed industry and also in the enzymatic pretreatment of biomass for feedstock and ethanol production.
宏基因组学已被广泛应用于发现新的酶和途径,以将木质纤维素生物质转化为燃料和化学品。在这种情况下,本研究报告了一种新型内切木聚糖酶家族 GH10(SCXyl)的分离、重组表达、生化和结构特征,该酶是从甘蔗土壤宏基因组中鉴定出来的。重组 SCXyl 对来自山毛榉木的木聚糖具有很高的活性,在 pH6.0 和 45°C 时表现出最佳的酶活性。晶体结构解析分辨率为 2.75Å,揭示了典型的(β/α)8-桶折叠结构,具有保守的活性口袋和色氨酸 281-精氨酸 291 环的固有灵活性,该环可以根据底物结合采用不同的构象状态。降解产物的毛细管电泳分析表明,该酶显示出降解小的木寡糖(如木三糖)的异常能力,这与+1 亚位点的疏水性接触和远离水解位点的亚位点的低结合能一致。来自木聚糖聚合物和磷酸预处理甘蔗渣(PASB)的主要反应产物是木寡糖,但在更长的孵育时间后,也形成了木二糖和木糖。此外,在添加商业纤维素酶混合物之前,将 SCXyl 用作 PASB 的预处理步骤,显著增强了糖化过程。所有这些特性都证明了该酶在食品和饲料工业中的几个生物技术过程以及生物质的酶预处理用于原料和乙醇生产中的有利应用。