Laboratory of Toxicology and Pharmacology, National Institute of Environmental Health Sciences, National Institutes of Health, Research Triangle Park, North Carolina (B.K.S., A.K., S.B., R.P.M.); and National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland (M.G.E.).
J Pharmacol Exp Ther. 2013 Dec;347(3):607-14. doi: 10.1124/jpet.113.207928. Epub 2013 Sep 18.
Nitric oxide (·NO) was originally identified as an innate cytotoxin. However, in tumors it can enhance resistance to chemotherapy and exacerbate cancer progression. Our previous studies indicated that (·NO/·NO-derived species react with etoposide (VP-16) in vitro and form products that show significantly reduced activity toward HL60 cells and lipopolysaccharide (LPS)-induced macrophages. Here, we further confirm the hypothesis that (÷)NO generation contributes to VP-16 resistance by examining interactions of ·NO with VP-16 in inducible nitric-oxide synthase (iNOS)-expressing human melanoma A375 cells. Inhibition of iNOS catalysis by N(6)-(1-iminoethyl)-L-lysine dihydrochloride (L-NIL) in human melanoma A375 cells reversed VP-16 resistance, leading to increased DNA damage and apoptosis. Furthermore, we found that coculturing A375 melanoma cells with LPS-induced macrophage RAW cells also significantly reduced VP-16 cytotoxicity and DNA damage in A375 cells. We also examined the interactions of (·)NO with another topoisomerase active drug, Adriamycin, in A375 cells. In contrast, to VP-16, (·)NO caused no significant modulation of cytotoxicity or Adriamycin-dependent apoptosis, suggesting that (⋅)NO does not interact with Adriamycin. Our studies support the hypothesis that (·)NO oxidative chemistry can detoxify VP-16 through direct nitrogen oxide radical attack. Our results provide insights into the pharmacology and anticancer mechanisms of VP-16 that may ultimately contribute to increased resistance, treatment failure, and induction of secondary leukemia in VP-16-treated patients.
一氧化氮(·NO)最初被鉴定为一种天然细胞毒素。然而,在肿瘤中,它可以增强对化疗的抵抗力并加剧癌症的进展。我们之前的研究表明,(·NO/·NO 衍生的物质在体外与依托泊苷(VP-16)反应,形成对 HL60 细胞和脂多糖(LPS)诱导的巨噬细胞活性显著降低的产物。在这里,我们通过检查·NO 与诱导型一氧化氮合酶(iNOS)表达的人黑色素瘤 A375 细胞中 VP-16 的相互作用,进一步证实了·NO 生成有助于 VP-16 耐药的假设。N(6)-(1-亚氨基乙基)-L-赖氨酸二盐酸盐(L-NIL)抑制人黑色素瘤 A375 细胞中 iNOS 催化作用,逆转 VP-16 耐药性,导致 DNA 损伤和细胞凋亡增加。此外,我们发现 A375 黑色素瘤细胞与 LPS 诱导的巨噬细胞 RAW 细胞共培养也显著降低了 A375 细胞中 VP-16 的细胞毒性和 DNA 损伤。我们还检查了(·)NO 与另一种拓扑异构酶活性药物阿霉素在 A375 细胞中的相互作用。与 VP-16 相反,(·)NO 对细胞毒性或阿霉素依赖性细胞凋亡没有显著调节作用,这表明(·)NO 与阿霉素没有相互作用。我们的研究支持(·)NO 氧化化学可以通过直接氮氧化物自由基攻击来解毒 VP-16 的假设。我们的结果为 VP-16 的药理学和抗癌机制提供了新的认识,这可能最终导致 VP-16 治疗患者的耐药性增加、治疗失败和继发性白血病的诱导。