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生物质燃烧对加纳萨凡纳地区纳武鲁空气质量的影响。

Biomass burning contribution to ambient air particulate levels at Navrongo in the Savannah zone of Ghana.

机构信息

National Nuclear Research Institute, Ghana Atomic Energy Commission, Legon, Accra, Ghana.

出版信息

J Air Waste Manag Assoc. 2013 Sep;63(9):1036-45. doi: 10.1080/10962247.2013.783888.

DOI:10.1080/10962247.2013.783888
PMID:24151679
Abstract

The concentrations of airborne particulate matter (PM) in Navrongo, a town in the Sahel Savannah Zone of Ghana, have been measured and the major sources have been identified. This area is prone to frequent particulate pollution episodes due to Harmattan dust and biomass burning, mostly from annual bushfires. The contribution of combustion emissions, particularly from biomass and fossil fuel, to ambient air particulate loadings was assessed. Sampling was conducted from February 2009 to February 2010 in Navrongo. Two Gent samplers were equipped to collect PM10 in two size fractions, coarse (PM10-2.5) and fine (PM2.5). Coarse particles are collected on a coated, 8-microm-pore Nuclepore filter. Fine particle samples were sampled with 47-mm-diameter Nuclepore and quartz filters. Elemental carbon (EC) and organic carbon (OC) concentrations were determined from the quartz filters using thermal optical reflectance (IMPROVE/TOR) methods. Elements were measured on the fine-particle Nuclepore filters using energy-dispersive x-ray fluorescence. The average PM2.5 mass concentration obtained at Navrongo was 32.3 microg/m. High carbonaceous concentrations were obtained from November to March, the period of Harmattan dust and severe bush fires. Total carbon was found to contribute approximately 40% of the PM2.5 particulate mass. Positive matrix factorization (PMF) suggested six major sources contributing to the PM2.5 mass. They are two stroke engines, gasoline emissions, soil dust, diesel emissions, biomass burning, and resuspended soil dust. Biomass combustion (16.0%) was identified as second most important source next to soil dust at Navrongo.

摘要

加纳萨赫勒草原区城镇纳瓦罗戈的空气中颗粒物(PM)浓度已经过测量,主要来源也已经确定。由于哈马丹尘暴和生物质燃烧,主要是每年的丛林大火,该地区经常发生颗粒物污染事件。评估了燃烧排放物,特别是生物质和化石燃料对环境空气中颗粒物负荷的贡献。采样于 2009 年 2 月至 2010 年 2 月在纳瓦罗戈进行。两台 Gent 采样器配备了两个大小分级,粗(PM10-2.5)和细(PM2.5),用于收集 PM10。粗颗粒收集在涂覆的 8 微米孔 Nuclepore 过滤器上。细颗粒样品使用 47 毫米直径的 Nuclepore 和石英过滤器进行采样。使用热光反射(IMPROVE/TOR)方法从石英过滤器中测定元素碳(EC)和有机碳(OC)浓度。使用能量色散 X 射线荧光法在细颗粒 Nuclepore 过滤器上测量元素。纳瓦罗戈的 PM2.5 质量浓度平均值为 32.3 微克/立方米。11 月至 3 月,哈马丹尘暴和严重丛林大火期间,获得了高碳浓度。总碳被发现对 PM2.5 颗粒物质量的贡献约为 40%。正矩阵因子化(PMF)表明,有六个主要来源对 PM2.5 质量有贡献。它们是二冲程发动机、汽油排放、土壤尘埃、柴油排放、生物质燃烧和再悬浮土壤尘埃。在纳瓦罗戈,生物质燃烧(16.0%)被确定为仅次于土壤尘埃的第二大重要来源。

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