Kim Ji-Hee, Noe G Timothy, McGill Stephen A, Wang Yongrui, Wójcik Aleksander K, Belyanin Alexey A, Kono Junichiro
Departments of Electrical & Computer Engineering and Physics & Astronomy, Rice University, Houston, TX 77005, USA.
Sci Rep. 2013 Nov 21;3:3283. doi: 10.1038/srep03283.
Nonequilibrium can be a source of order. This rather counterintuitive statement has been proven to be true through a variety of fluctuation-driven, self-organization behaviors exhibited by out-of-equilibrium, many-body systems in nature (physical, chemical, and biological), resulting in the spontaneous appearance of macroscopic coherence. Here, we report on the observation of spontaneous bursts of coherent radiation from a quantum-degenerate gas of nonequilibrium electron-hole pairs in semiconductor quantum wells. Unlike typical spontaneous emission from semiconductors, which occurs at the band edge, the observed emission occurs at the quasi-Fermi edge of the carrier distribution. As the carriers are consumed by recombination, the quasi-Fermi energy goes down toward the band edge, and we observe a continuously red-shifting streak. We interpret this emission as cooperative spontaneous recombination of electron-hole pairs, or superfluorescence (SF), which is enhanced by Coulomb interactions near the Fermi edge. This novel many-body enhancement allows the magnitude of the spontaneously developed macroscopic polarization to exceed the maximum value for ordinary SF, making electron-hole SF even more "super" than atomic SF.
非平衡态可以成为有序的来源。这个相当违反直觉的陈述已通过自然界中(物理、化学和生物)非平衡多体系统所展现的各种涨落驱动的自组织行为被证明是正确的,这些行为导致宏观相干性的自发出现。在此,我们报告了在半导体量子阱中非平衡电子 - 空穴对的量子简并气体中观察到的相干辐射的自发爆发。与典型的半导体自发发射(发生在能带边缘)不同,观察到的发射发生在载流子分布的准费米边缘。随着载流子通过复合被消耗,准费米能量向能带边缘下降,并且我们观察到一条持续红移的条纹。我们将这种发射解释为电子 - 空穴对的协同自发复合,即超荧光(SF),它在费米边缘附近通过库仑相互作用得到增强。这种新颖的多体增强使得自发产生的宏观极化幅度超过普通超荧光的最大值,使得电子 - 空穴超荧光比原子超荧光更具“超”性。