Ding Cairong, Lv Zesheng, Zeng Xueran, Zhang Baijun
State Key Laboratory of Optoelectronic Materials and Technologies, School of Electronics and Information Technology (School of Microelectronics), Sun Yat-sen University, Guangzhou 510275, China.
Nanomaterials (Basel). 2022 Jan 20;12(3):327. doi: 10.3390/nano12030327.
Superfluorescence is a collective emission from quantum coherent emitters due to quantum fluctuations. This is characterized by the existence of the delay time (τD) for the emitters coupling and phase-synchronizing to each other spontaneously. Here we report the observation of superfluorescence in c-plane InGaN/GaN multiple-quantum wells by time-integrated and time-resolved photoluminescence spectroscopy under higher excitation fluences of the 267 nm laser and at room temperature, showing a characteristic τD from 79 ps to 62 ps and the ultrafast radiative decay (7.5 ps) after a burst of photons. Time-resolved traces present a small quantum oscillation from coupled InGaN/GaN multiple-quantum wells. The superfluorescence is attributed to the radiative recombination of coherent emitters distributing on strongly localized subband states, → or → in 3nm width multiple-quantum wells. Our work paves the way for deepening the understanding of the emission mechanism in the InGaN/GaN quantum well at a higher injected carrier density.
超荧光是量子相干发射体由于量子涨落而产生的集体发射。其特征在于发射体之间自发耦合和相位同步存在延迟时间(τD)。在此,我们报告在室温下,利用时间积分和时间分辨光致发光光谱,在267nm激光的较高激发通量下,观测到c面InGaN/GaN多量子阱中的超荧光,其特征延迟时间从79皮秒到62皮秒,并且在一阵光子发射后呈现超快辐射衰减(7.5皮秒)。时间分辨轨迹显示出耦合的InGaN/GaN多量子阱存在小的量子振荡。超荧光归因于分布在3nm宽度多量子阱中强局域子带态上的相干发射体的辐射复合。我们的工作为在更高注入载流子密度下加深对InGaN/GaN量子阱发射机制的理解铺平了道路。