Song Wooseok, Kwon Soon Yeol, Myung Sung, Jung Min Wook, Kim Seong Jun, Min Bok Ki, Kang Min-A, Kim Sung Ho, Lim Jongsun, An Ki-Seok
Thin Film Materials Research Group, Korea Research Institute of Chemical Technology (KRICT), Yuseong P. O. Box 107, Daejeon 305-600, Republic of Korea.
Sci Rep. 2014 Feb 11;4:4064. doi: 10.1038/srep04064.
In order to combine advantages of ZnO thin film transistors (TFTs) with a high on-off ratio and graphene TFTs with extremely high carrier mobility, we present a facile methodology for fabricating ZnO thin film/graphene hybrid two-dimensional TFTs. Hybrid TFTs exhibited ambipolar behavior, an outstanding electron mobility of 329.7 ± 16.9 cm(2)/V·s, and a high on-off ratio of 10(5). The ambipolar behavior of the ZnO/graphene hybrid TFT with high electron mobility could be due to the superimposed density of states involving the donor states in the bandgap of ZnO thin films and the linear dispersion of monolayer graphene. We further established an applicable circuit model for understanding the improvement in carrier mobility of ZnO/graphene hybrid TFTs.
为了将具有高开/关比的氧化锌薄膜晶体管(TFT)的优势与具有极高载流子迁移率的石墨烯TFT的优势相结合,我们提出了一种用于制造氧化锌薄膜/石墨烯混合二维TFT的简便方法。混合TFT表现出双极性行为、329.7±16.9 cm²/V·s的出色电子迁移率以及10⁵的高开/关比。具有高电子迁移率的氧化锌/石墨烯混合TFT的双极性行为可能归因于氧化锌薄膜带隙中施主态的态密度叠加以及单层石墨烯的线性色散。我们进一步建立了一个适用的电路模型,以理解氧化锌/石墨烯混合TFT载流子迁移率的提高。