Center for Soft Matter Research, New York University, 4 Washington Place, New York, New York 10003, USA.
SUPA, School of Physics and Astronomy, University of Edinburgh, JCMB Kings Buildings, Mayfield Road, Edinburgh EH9 3JZ, United Kingdom.
Phys Rev Lett. 2014 Mar 7;112(9):098302. doi: 10.1103/PhysRevLett.112.098302. Epub 2014 Mar 6.
A consensus is emerging that discontinuous shear thickening (DST) in dense suspensions marks a transition from a flow state where particles remain well separated by lubrication layers, to one dominated by frictional contacts. We show here that reasonable assumptions about contact proliferation predict two distinct types of DST in the absence of inertia. The first occurs at densities above the jamming point of frictional particles; here, the thickened state is completely jammed and (unless particles deform) cannot flow without inhomogeneity or fracture. The second regime shows strain-rate hysteresis and arises at somewhat lower densities, where the thickened phase flows smoothly. DST is predicted to arise when finite-range repulsions defer contact formation until a characteristic stress level is exceeded.
人们越来越认为,在密集悬浮液中不连续剪切增稠(DST)标志着从一个流动状态向一个由摩擦接触主导的状态的转变,在这个流动状态中,颗粒通过润滑层保持良好的分离。我们在这里表明,关于接触增殖的合理假设可以预测在没有惯性的情况下 DST 的两种不同类型。第一种情况发生在摩擦颗粒的堵塞点以上的密度下;在这种情况下,增稠状态完全堵塞,除非颗粒变形,否则在没有不均匀性或断裂的情况下无法流动。第二个区域显示应变率滞后,并且出现在密度稍低的地方,在那里增稠相可以平滑地流动。当有限范围的斥力推迟接触形成直到超过特征应力水平时,预计会出现 DST。