Lam Pui Ying, Zhu Fu-Yuan, Chan Wai Lung, Liu Hongjia, Lo Clive
School of Biological Sciences, The University of Hong Kong, Pokfulam, Hong Kong, China (P.Y.L., F.-Y.Z., W.L.C., C.L.); andState Key Laboratory Breeding Base for Zhejiang Sustainable Pest and Disease Control, Institute of Crops and Nuclear Technology Utilization, Zhejiang Academy of Agricultural Sciences, Hangzhou 310021, China (H.L.).
School of Biological Sciences, The University of Hong Kong, Pokfulam, Hong Kong, China (P.Y.L., F.-Y.Z., W.L.C., C.L.); andState Key Laboratory Breeding Base for Zhejiang Sustainable Pest and Disease Control, Institute of Crops and Nuclear Technology Utilization, Zhejiang Academy of Agricultural Sciences, Hangzhou 310021, China (H.L.)
Plant Physiol. 2014 Jul;165(3):1315-1327. doi: 10.1104/pp.114.239723. Epub 2014 May 19.
Flavones are a major class of flavonoids with a wide range of physiological functions in plants. They are constitutively accumulated as C-glycosides and O-linked conjugates in vegetative tissues of grasses. It has long been presumed that the two structural modifications of flavones occur through independent metabolic routes. Previously, we reported that cytochrome P450 93G2 (CYP93G2) functions as a flavanone 2-hydroxylase (F2H) that provides 2-hydroxyflavanones for C-glycosylation in rice (Oryza sativa). Flavone C-glycosides are subsequently formed by dehydratase activity on 2-hydroxyflavanone C-glycosides. On the other hand, O-linked modifications were proposed to proceed after the flavone nucleus is generated. In this study, we demonstrate that CYP93G1, the closest homolog of CYP93G2 in rice, is a bona fide flavone synthase II (FNSII) that catalyzes the direct conversion of flavanones to flavones. In recombinant enzyme assays, CYP93G1 desaturated naringenin and eriodictyol to apigenin and luteolin, respectively. Consistently, transgenic expression of CYP93G1 in Arabidopsis (Arabidopsis thaliana) resulted in the accumulation of different flavone O-glycosides, which are not naturally present in cruciferous plants. Metabolite analysis of a rice CYP93G1 insertion mutant further demonstrated the preferential depletion of tricin O-linked flavanolignans and glycosides. By contrast, redirection of metabolic flow to the biosynthesis of flavone C-glycosides was observed. Our findings established that CYP93G1 is a key branch point enzyme channeling flavanones to the biosynthesis of tricin O-linked conjugates in rice. Functional diversification of F2H and FNSII in the cytochrome P450 CYP93G subfamily may represent a lineage-specific event leading to the prevalent cooccurrence of flavone C- and O-linked derivatives in grasses today.
黄酮类化合物是一类主要的黄酮,在植物中具有广泛的生理功能。它们以C-糖苷和O-连接的共轭物形式组成性地积累在禾本科植物的营养组织中。长期以来,人们一直认为黄酮的两种结构修饰是通过独立的代谢途径发生的。此前,我们报道细胞色素P450 93G2(CYP93G2)作为黄烷酮2-羟化酶(F2H)发挥作用,为水稻(Oryza sativa)中的C-糖基化提供2-羟基黄烷酮。黄酮C-糖苷随后通过2-羟基黄烷酮C-糖苷的脱水酶活性形成。另一方面,有人提出O-连接修饰在黄酮核生成后进行。在本研究中,我们证明CYP93G1是水稻中CYP93G2最接近的同源物,是一种真正的黄酮合酶II(FNSII),可催化黄烷酮直接转化为黄酮。在重组酶测定中,CYP93G1分别将柚皮素和圣草酚去饱和为芹菜素和木犀草素。一致地,CYP93G1在拟南芥(Arabidopsis thaliana)中的转基因表达导致不同黄酮O-糖苷的积累,这些黄酮O-糖苷在十字花科植物中并非天然存在。水稻CYP93G1插入突变体的代谢物分析进一步证明了小麦黄素O-连接的黄烷醇木脂素和糖苷优先消耗。相比之下,观察到代谢流转向黄酮C-糖苷的生物合成。我们的研究结果表明,CYP93G1是水稻中引导黄烷酮进入小麦黄素O-连接共轭物生物合成的关键分支点酶。细胞色素P450 CYP93G亚家族中F2H和FNSII的功能多样化可能代表了一个谱系特异性事件,导致如今黄酮C-和O-连接衍生物在禾本科植物中普遍共存。