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Breakthroughs in hard X-ray diffraction: towards a multiscale science approach in heterogeneous catalysis.

作者信息

Ristanović Zoran, Weckhuysen Bert M

机构信息

Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht (The Netherlands).

出版信息

Angew Chem Int Ed Engl. 2014 Aug 11;53(33):8556-8. doi: 10.1002/anie.201404463. Epub 2014 Jul 2.

DOI:10.1002/anie.201404463
PMID:24990145
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC4834627/
Abstract

: Modern heterogeneous catalysis would benefit from a multiscale science approach bridging the molecular world with the macroscopic world. Because of recent breakthroughs in X‐ray diffraction methods, including the surface X‐ray diffraction of atomically flat model catalysts, X‐ray diffraction tomography of catalyst bodies, and X‐ray profiling of an active catalyst in a chemical reactor, such an approach is now within reach.[Image: see text]

摘要
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c89/4834627/794113cf462c/ANIE-53-8556-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c89/4834627/794113cf462c/ANIE-53-8556-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c89/4834627/794113cf462c/ANIE-53-8556-g001.jpg

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本文引用的文献

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Dazzling history.辉煌的历史。
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High-energy surface X-ray diffraction for fast surface structure determination.用于快速表面结构测定的高能表面 X 射线衍射。
Science. 2014 Feb 14;343(6172):758-61. doi: 10.1126/science.1246834. Epub 2014 Jan 30.
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X-ray science: The big guns.X射线科学：强大武器。
Nature. 2014 Jan 30;505(7485):604-6. doi: 10.1038/505604a.
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Crystallography: Atomic secrets.晶体学：原子奥秘。
Nature. 2014 Jan 30;505(7485):602-3. doi: 10.1038/505602a.
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Pair distribution function computed tomography.配对分布函数计算机断层扫描。
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Watching the methanol-to-olefin process with time- and space-resolved high-energy operando X-ray diffraction.利用具有时间和空间分辨能力的高能原位X射线衍射观察甲醇制烯烃过程。
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