National Center for Atmospheric Research, Boulder, Colorado 80301, United States.
Environ Sci Technol. 2014 Aug 19;48(16):9523-30. doi: 10.1021/es502250z. Epub 2014 Jul 28.
The open burning of waste, whether at individual residences, businesses, or dump sites, is a large source of air pollutants. These emissions, however, are not included in many current emission inventories used for chemistry and climate modeling applications. This paper presents the first comprehensive and consistent estimates of the global emissions of greenhouse gases, particulate matter, reactive trace gases, and toxic compounds from open waste burning. Global emissions of CO2 from open waste burning are relatively small compared to total anthropogenic CO2; however, regional CO2 emissions, particularly in many developing countries in Asia and Africa, are substantial. Further, emissions of reactive trace gases and particulate matter from open waste burning are more significant on regional scales. For example, the emissions of PM10 from open domestic waste burning in China is equivalent to 22% of China's total reported anthropogenic PM10 emissions. The results of the emissions model presented here suggest that emissions of many air pollutants are significantly underestimated in current inventories because open waste burning is not included, consistent with studies that compare model results with available observations.
废物露天燃烧,无论是在个人住宅、企业还是垃圾场,都是空气污染物的一大来源。然而,在许多用于化学和气候建模应用的现行排放清单中,并未将这些排放物包括在内。本文首次全面而一致地估算了全球温室气体、颗粒物、活性痕量气体和有毒化合物因露天废物燃烧而产生的排放量。与人为 CO2 排放总量相比,露天废物燃烧产生的 CO2 排放量相对较小;然而,特别是在亚洲和非洲的许多发展中国家,区域 CO2 排放量相当可观。此外,活性痕量气体和颗粒物因露天废物燃烧而产生的排放量在区域范围内更为显著。例如,中国露天燃烧城市生活垃圾所产生的 PM10 排放量相当于中国报告的人为 PM10 排放量的 22%。这里提出的排放模型的结果表明,由于未将露天废物燃烧包括在内,目前的排放清单大大低估了许多空气污染物的排放量,这与将模型结果与现有观测结果进行比较的研究结果一致。