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通过模式展开解释单个 V-天线的定向荧光发射。

Directional fluorescence emission by individual V-antennas explained by mode expansion.

出版信息

ACS Nano. 2014 Aug 26;8(8):8232-41. doi: 10.1021/nn502616k.

Abstract

Specially designed plasmonic antennas can, by far-field interference of different antenna elements or a combination of multipolar antenna modes, scatter light unidirectionally, allowing for directional light control at the nanoscale. One of the most basic and compact geometries for such antennas is a nanorod with broken rotational symmetry, in the shape of the letter V. In this article, we show that these V-antennas unidirectionally scatter the emission of a local dipole source in a direction opposite the undirectional side scattering of a plane wave. Moreover, we observe high directivity, up to 6 dB, only for certain well-defined positions of the emitter relative to the antenna. By employing a rigorous eigenmode expansion analysis of the V-antenna, we fully elucidate the fundamental origin of its directional behavior. All findings are experimentally verified by measuring the radiation patterns of a scattered plane wave and the emission pattern of fluorescently doped PMMA positioned in different regions around the antenna. The fundamental interference effects revealed in the eigenmode expansion can serve as guidelines in the understanding and further development of nanoscale directional scatterers.

摘要

特别设计的等离子体天线可以通过不同天线元件的远场干涉或多极天线模式的组合,单向散射光,从而实现纳米尺度的光的定向控制。对于这种天线,最基本和紧凑的几何形状之一是具有非旋转对称性的纳米棒,形状为字母 V。在本文中,我们表明这些 V 型天线在与平面波的单向散射相反的方向上单向散射局部偶极子源的发射。此外,我们观察到只有在发射器相对于天线的某些定义明确的位置时,才会出现高达 6dB 的高指向性。通过对 V 型天线的本征模展开分析,我们充分阐明了其定向行为的基本原理。所有发现都通过测量散射平面波的辐射模式和荧光掺杂 PMMA 在天线周围不同区域的发射模式来实验验证。本征模展开中揭示的基本干涉效应可以作为理解和进一步开发纳米尺度定向散射体的指南。

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