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单等离子体散射体的定向发射。

Directional emission from a single plasmonic scatterer.

机构信息

Center for Nanophotonics, FOM Institute AMOLF, Science Park 104, 1098 XG Amsterdam, The Netherlands.

出版信息

Nat Commun. 2014;5:3250. doi: 10.1038/ncomms4250.

Abstract

Directing light emission is key for many applications in photonics and biology. Optical antennas made from nanostructured plasmonic metals are suitable candidates for this purpose but designing antennas with good directional characteristics can be challenging, especially when they consist of multiple elements. Here we show that strongly directional emission can also be obtained from a simple individual gold nanodisk, utilizing the far-field interference of resonant electric and magnetic modes. Using angle-resolved cathodoluminescence spectroscopy, we find that the spectral and angular response strongly depends on excitation position. For excitation at the nanodisk edge, interference between in-plane and out-of-plane dipole components leads to strong beaming of light. For large nanodisks, higher-order multipole components contribute significantly to the scattered field, leading to enhanced directionality. Using a combination of full-wave simulations and analytical point scattering theory we are able to decompose the calculated and measured scattered fields into dipolar and quadrupolar contributions.

摘要

引导光发射是光子学和生物学中许多应用的关键。由纳米结构等离子体金属制成的光学天线是实现这一目的的合适候选者,但设计具有良好方向性特征的天线可能具有挑战性,特别是当它们由多个元件组成时。在这里,我们展示了利用共振电场和磁场模式的远场干涉,也可以从简单的单个金纳米盘获得强烈的定向发射。使用角度分辨的阴极发光光谱学,我们发现光谱和角度响应强烈依赖于激发位置。对于在纳米盘边缘的激发,平面内和平面外偶极分量之间的干涉导致光的强烈定向发射。对于较大的纳米盘,高阶多极分量对散射场有显著贡献,从而提高了方向性。我们使用全波模拟和分析点散射理论的组合,将计算和测量的散射场分解为偶极子和四极子贡献。

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