Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University , Singapore 637371.
Nano Lett. 2014 Oct 8;14(10):5995-6001. doi: 10.1021/nl503057g. Epub 2014 Sep 10.
Near-infrared (NIR) solid-state micro/nanolasers are important building blocks for true integration of optoelectronic circuitry. Although significant progress has been made in III-V nanowire lasers with achieving NIR lasing at room temperature, challenges remain including low quantum efficiencies and high Auger losses. Importantly, the obstacles toward integrating one-dimensional nanowires on the planar ubiquitous Si platform need to be effectively tackled. Here we demonstrate a new family of planar room-temperature NIR nanolasers based on organic-inorganic perovskite CH3NH3PbI(3-a)X(a) (X = I, Br, Cl) nanoplatelets. Their large exciton binding energies, long diffusion lengths, and naturally formed high-quality planar whispering-gallery mode cavities ensure adequate gain and efficient optical feedback for low-threshold optically pumped in-plane lasing. We show that these remarkable wavelength tunable whispering-gallery nanolasers can be easily integrated onto conductive platforms (Si, Au, indium tin oxide, and so forth). Our findings open up a new class of wavelength tunable planar nanomaterials potentially suitable for on-chip integration.
近红外(NIR)固态微/纳米激光器是实现光电电路真正集成的重要组成部分。尽管 III-V 纳米线激光器在实现室温 NIR 激光方面已经取得了重大进展,但仍存在一些挑战,包括量子效率低和俄歇损耗高。重要的是,需要有效地解决将一维纳米线集成到平面无处不在的 Si 平台上的障碍。在这里,我们展示了一类基于有机-无机钙钛矿 CH3NH3PbI(3-a)X(a)(X = I、Br、Cl)纳米板的新型平面室温 NIR 纳米激光器。它们具有较大的激子结合能、较长的扩散长度和自然形成的高质量平面 whispering-gallery 模式腔,确保了低阈值光泵浦面内激光的足够增益和有效的光学反馈。我们表明,这些显著的波长可调 whispering-gallery 纳米激光器可以很容易地集成到导电平台(Si、Au、氧化铟锡等)上。我们的发现开辟了一类新的波长可调谐平面纳米材料,它们可能适合于芯片集成。