Wang Zi-Wu, Li Zhi-Qing, Li Shu-Shen
Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing Technology, Department of Physics, Tianjin University, Tianjin 300072, People's Republic of China.
J Phys Condens Matter. 2014 Oct 1;26(39):395302. doi: 10.1088/0953-8984/26/39/395302. Epub 2014 Sep 5.
In the frame of Huang-Rhys's lattice relaxation model, we theoretically investigate the electron relaxation assisted by optical phonon resonance scattering among Landau levels with spin-conserving and spin-flip processes in graphene. We not only consider the longitudinal optical (LO) phonon scattering, but also the surface optical (SO) phonon scattering induced by the polar substrate under the graphene. The relaxation rate displays a Gaussian distribution by considering the effect of lattice relaxation that arises from the electron-deformation potential acoustic phonon interaction. We find that the relaxation rate of the spin-conserving process is three orders of magnitude larger than that of the spin-flip process for the same phonon mode. Moreover, the discrepancy of relaxation rates between the SO and LO phonon scattering is at two orders of magnitude for the same process. The opposite temperature dependence of the relaxation rates are also obtained in the resonance energy regime in the present model. In addition, the influences of the strength of Rashba spin-orbital coupling, the dielectric constant of different polar substrates and the distance between the graphene and substrate on the relaxation rates are also discussed quantitatively for the SO phonon scattering. The obtained results could be useful for the graphene-based applications on the mid-infrared and terahertz modulation and spintronic devices.
在黄-里斯晶格弛豫模型的框架下,我们从理论上研究了石墨烯中朗道能级间光学声子共振散射辅助的电子弛豫过程,包括自旋守恒和自旋翻转过程。我们不仅考虑了纵向光学(LO)声子散射,还考虑了石墨烯下方极性衬底诱导的表面光学(SO)声子散射。通过考虑由电子-形变势声学声子相互作用引起的晶格弛豫效应,弛豫率呈现高斯分布。我们发现,对于相同的声子模式,自旋守恒过程的弛豫率比自旋翻转过程的弛豫率大三个数量级。此外,对于相同的过程,SO声子散射和LO声子散射的弛豫率差异在两个数量级。在本模型的共振能量区域,还得到了弛豫率相反的温度依赖性。此外,还定量讨论了拉什巴自旋-轨道耦合强度、不同极性衬底的介电常数以及石墨烯与衬底之间的距离对SO声子散射弛豫率的影响。所得结果对于基于石墨烯的中红外和太赫兹调制以及自旋电子器件应用可能是有用的。