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中国宣威和富源县女性人群中固体燃料燃烧导致的家庭空气污染中的多环芳烃暴露。

Polycyclic aromatic hydrocarbon exposure in household air pollution from solid fuel combustion among the female population of Xuanwei and Fuyuan counties, China.

作者信息

Downward George S, Hu Wei, Rothman Nat, Reiss Boris, Wu Guoping, Wei Fusheng, Chapman Robert S, Portengen Lutzen, Qing Lan, Vermeulen Roel

机构信息

Institute for Risk Assessment Sciences, Division of Environmental Epidemiology, Utrecht University , Utrecht 3512 JE, The Netherlands.

出版信息

Environ Sci Technol. 2014 Dec 16;48(24):14632-41. doi: 10.1021/es504102z. Epub 2014 Nov 21.

Abstract

Exposure to polycyclic aromatic hydrocarbons (PAHs) from burning "smoky" (bituminous) coal has been implicated as a cause of the high lung cancer incidence in the counties of Xuanwei and Fuyuan, China. Little is known about variations in PAH exposure from throughout the region nor how fuel source and stove design affects exposure. Indoor and personal PAH exposure resulting from solid fuel combustion in Xuanwei and Fuyuan was investigated using repeated 24 h particle bound and gas-phase PAH measurements, which were collected from 163 female residents of Xuanwei and Fuyuan. 549 particle bound (283 indoor and 266 personal) and 193 gas phase (all personal) PAH measurements were collected. Mixed effect models indicated that PAH exposure was up to 6 times higher when burning smoky coal than smokeless coal and varied by up to a factor of 3 between different smoky coal geographic sources. PAH measurements from unventilated firepits were up to 5 times that of ventilated stoves. Exposure also varied between different room sizes and season of measurement. These findings indicate that PAH exposure is modulated by a variety of factors, including fuel type, coal source, and stove design. These findings may provide valuable insight into potential causes of lung cancer in the area.

摘要

在中国宣威和富源地区,因燃烧“冒烟”(烟煤)煤而接触多环芳烃(PAHs)被认为是该地区肺癌高发的一个原因。对于整个地区PAH暴露的差异以及燃料来源和炉灶设计如何影响暴露情况,人们了解甚少。通过对宣威和富源163名女性居民进行重复的24小时颗粒结合态和气态PAH测量,研究了固体燃料燃烧导致的室内和个人PAH暴露情况。共收集了549次颗粒结合态(283次室内和266次个人)和193次气相(均为个人)PAH测量数据。混合效应模型表明,燃烧烟煤时的PAH暴露比燃烧无烟煤时高出多达6倍,并且在不同的烟煤地理来源之间变化高达3倍。未通风火坑的PAH测量值高达通风炉灶的5倍。暴露情况在不同房间大小和测量季节之间也有所不同。这些发现表明,PAH暴露受到多种因素的调节,包括燃料类型、煤源和炉灶设计。这些发现可能为该地区肺癌的潜在病因提供有价值的见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/477a/4270388/ae62e73be88d/es-2014-04102z_0001.jpg

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