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非布朗悬浮液中不同的粘度和软颗粒流变学

Diverging viscosity and soft granular rheology in non-Brownian suspensions.

作者信息

Kawasaki Takeshi, Coslovich Daniele, Ikeda Atsushi, Berthier Ludovic

机构信息

Laboratoire Charles Coulomb, UMR 5221, CNRS and Université Montpellier 2, Montpellier, France.

Fukui Institute for Fundamental Chemistry, Kyoto University, Kyoto, Japan.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Jan;91(1):012203. doi: 10.1103/PhysRevE.91.012203. Epub 2015 Jan 26.

Abstract

We use large scale computer simulations and finite-size scaling analysis to study the shear rheology of dense three-dimensional suspensions of frictionless non-Brownian particles in the vicinity of the jamming transition. We perform simulations of soft repulsive particles at constant shear rate, constant pressure, and finite system size and carefully study the asymptotic limits of large system sizes and infinitely hard particle repulsion. We first focus on the asymptotic behavior of the shear viscosity in the hard particle limit. By measuring the viscosity increase over about 5 orders of magnitude, we are able to confirm its asymptotic power law divergence close to the jamming transition. However, a precise determination of the critical density and critical exponent is difficult due to the "multiscaling" behavior of the viscosity. Additionally, finite-size scaling analysis suggests that this divergence is accompanied by a growing correlation length scale, which also diverges algebraically. Finally, we study the effect of particle softness and propose a natural extension of the standard granular rheology, which we test against our simulation data. Close to the jamming transition, this "soft granular rheology" offers a detailed description of the nonlinear rheology of soft particles, which differs from earlier empirical scaling forms.

摘要

我们使用大规模计算机模拟和有限尺寸标度分析来研究无摩擦非布朗粒子的密集三维悬浮液在堵塞转变附近的剪切流变学。我们在恒定剪切速率、恒定压力和有限系统尺寸下对软排斥粒子进行模拟,并仔细研究大系统尺寸和无限硬粒子排斥的渐近极限。我们首先关注硬粒子极限下剪切粘度的渐近行为。通过测量约5个数量级的粘度增加,我们能够确认其在堵塞转变附近的渐近幂律发散。然而,由于粘度的“多标度”行为,精确确定临界密度和临界指数很困难。此外,有限尺寸标度分析表明,这种发散伴随着不断增长的关联长度尺度,该尺度也代数发散。最后,我们研究了粒子柔软度的影响,并提出了标准颗粒流变学的自然扩展,我们根据模拟数据对其进行了测试。在堵塞转变附近,这种“软颗粒流变学”提供了软粒子非线性流变学的详细描述,这与早期的经验标度形式不同。

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