Wang Fenglin, Stepanov Petr, Gray Mason, Lau Chun Ning
Department of Physics and Astronomy, University of California, Riverside, CA 92521, USA.
Nanotechnology. 2015 Mar 13;26(10):105709. doi: 10.1088/0957-4484/26/10/105709. Epub 2015 Feb 20.
We fabricate suspended molybdenum disulfide (MoS2) field effect transistor devices and develop an effective gas annealing technique that significantly improves device quality and increases conductance by 3-4 orders of magnitude. Mobility of the suspended devices ranges from 0.01 to 46 cm(2) V(-1) s(-1) before annealing, and from 0.5 to 105 cm(2) V(-1) s(-1) after annealing. Temperature dependence measurements reveal two transport mechanisms: electron-phonon scattering at high temperatures and thermal activation over a gate-tunable barrier height at low temperatures. Our results suggest that transport in these devices is not limited by the substrates, but likely by defects, charge impurities and/or Schottky barriers at the metal-MoS2 interfaces. Finally, this suspended MoS2 device structure provides a versatile platform for other research areas, such as thermal, optical and mechanical studies.
我们制造了悬浮式二硫化钼(MoS2)场效应晶体管器件,并开发了一种有效的气体退火技术,该技术可显著提高器件质量,并使电导率提高3至4个数量级。悬浮器件在退火前的迁移率范围为0.01至46 cm² V⁻¹ s⁻¹,退火后的迁移率范围为0.5至105 cm² V⁻¹ s⁻¹。温度依赖性测量揭示了两种传输机制:高温下的电子-声子散射和低温下通过栅极可调势垒高度的热激活。我们的结果表明,这些器件中的传输不受衬底限制,而可能受金属-MoS2界面处的缺陷、电荷杂质和/或肖特基势垒限制。最后,这种悬浮式MoS2器件结构为其他研究领域,如热学、光学和力学研究,提供了一个通用平台。