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悬浮二硫化钼器件的退火与输运研究

Annealing and transport studies of suspended molybdenum disulfide devices.

作者信息

Wang Fenglin, Stepanov Petr, Gray Mason, Lau Chun Ning

机构信息

Department of Physics and Astronomy, University of California, Riverside, CA 92521, USA.

出版信息

Nanotechnology. 2015 Mar 13;26(10):105709. doi: 10.1088/0957-4484/26/10/105709. Epub 2015 Feb 20.

Abstract

We fabricate suspended molybdenum disulfide (MoS2) field effect transistor devices and develop an effective gas annealing technique that significantly improves device quality and increases conductance by 3-4 orders of magnitude. Mobility of the suspended devices ranges from 0.01 to 46 cm(2) V(-1) s(-1) before annealing, and from 0.5 to 105 cm(2) V(-1) s(-1) after annealing. Temperature dependence measurements reveal two transport mechanisms: electron-phonon scattering at high temperatures and thermal activation over a gate-tunable barrier height at low temperatures. Our results suggest that transport in these devices is not limited by the substrates, but likely by defects, charge impurities and/or Schottky barriers at the metal-MoS2 interfaces. Finally, this suspended MoS2 device structure provides a versatile platform for other research areas, such as thermal, optical and mechanical studies.

摘要

我们制造了悬浮式二硫化钼(MoS2)场效应晶体管器件,并开发了一种有效的气体退火技术,该技术可显著提高器件质量,并使电导率提高3至4个数量级。悬浮器件在退火前的迁移率范围为0.01至46 cm² V⁻¹ s⁻¹,退火后的迁移率范围为0.5至105 cm² V⁻¹ s⁻¹。温度依赖性测量揭示了两种传输机制:高温下的电子-声子散射和低温下通过栅极可调势垒高度的热激活。我们的结果表明,这些器件中的传输不受衬底限制,而可能受金属-MoS2界面处的缺陷、电荷杂质和/或肖特基势垒限制。最后,这种悬浮式MoS2器件结构为其他研究领域,如热学、光学和力学研究,提供了一个通用平台。

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