Department of Electrical Engineering and Computer Science, University of Michigan, Ann Arbor, MI 48109, USA.
Nanoscale. 2016 Apr 14;8(14):7755-60. doi: 10.1039/c5nr08954a.
Substantial effort has been dedicated to understand the intrinsic electronic properties of molybdenum disulfide (MoS2). However, electron transport study on monolayer MoS2 has been challenging to date, especially at low temperatures due to large metal/semiconductor junction barriers. Herein, we report the fabrication and characterization of the monolayer MoS2 single-electron transistor. High performance devices are obtained through the use of low work function metal (zinc) contact and a rapid thermal annealing step. Coulomb blockade is observed at low temperatures and is attributed to single-electron tunneling via two tunnel junction barriers. The nature of Coulomb blockade is also investigated by temperature-dependent conductance oscillation measurement. Our results hold promise for the study of novel quantum transport phenomena in 2D semiconducting atomic layer crystals.
人们投入了大量精力来理解二硫化钼(MoS2)的固有电子特性。然而,迄今为止,单层 MoS2 的电子输运研究一直具有挑战性,尤其是在低温下,这是由于大的金属/半导体结势垒造成的。在此,我们报告了单层 MoS2 单电子晶体管的制造和特性。通过使用低功函数金属(锌)接触和快速热退火步骤,获得了高性能器件。在低温下观察到库仑阻塞,这归因于通过两个隧道结势垒的单电子隧道。通过温度相关的电导振荡测量也研究了库仑阻塞的性质。我们的结果为研究二维半导体原子层晶体中的新型量子输运现象提供了希望。