Igarashi Jun-Ichi, Nagao Tatsuya
Faculty of Science, Ibaraki University, Mito, Ibaraki 310-8512, Japan.
J Phys Condens Matter. 2015 May 13;27(18):186002. doi: 10.1088/0953-8984/27/18/186002. Epub 2015 Apr 20.
We study the magnetic excitation spectra of resonant inelastic x-ray scattering (RIXS) at the L-edge from undoped cuprates beyond the fast collision approximation. We analyse the effect of the symmetry breaking ground state on the RIXS process of the Heisenberg model by using a projection procedure. We derive the expressions of the scattering amplitude in both one-magnon and two-magnon excitation channels. Each of them consists of the isotropic and anisotropic contributions. The latter is a new finding and attributed to the long range order of the ground state. The presence of anisotropic terms is supported by numerical calculations on a two-dimensional spin cluster. We express the RIXS spectra in the form of spin-correlation functions with the coefficients evaluated on the cluster, and calculate the function in a two dimensional system within the 1/S expansion. Due to the anisotropic terms, the spectral intensities are considerably enhanced around momentum transfer q = 0 in both one-magnon and two-magnon excitation channels. This finding may be experimentally confirmed by examining carefully the q-dependence of the spectra.
我们研究了未掺杂铜酸盐在L边的共振非弹性X射线散射(RIXS)的磁激发光谱,超越了快速碰撞近似。我们通过使用投影方法分析了对称破缺基态对海森堡模型RIXS过程的影响。我们推导了单磁振子和双磁振子激发通道中散射振幅的表达式。每个通道都由各向同性和各向异性贡献组成。后者是一个新发现,归因于基态的长程序。二维自旋簇的数值计算支持了各向异性项的存在。我们以自旋相关函数的形式表示RIXS光谱,其系数在簇上进行评估,并在1/S展开的二维系统中计算该函数。由于各向异性项,在单磁振子和双磁振子激发通道中,动量转移q = 0附近的光谱强度显著增强。通过仔细检查光谱的q依赖性,这一发现可能会得到实验证实。