Ho C M, Muthukumar V N, Ogata M, Anderson P W
Department of Applied Physics, University of Tokyo, Japan.
Phys Rev Lett. 2001 Feb 19;86(8):1626-9. doi: 10.1103/PhysRevLett.86.1626.
We investigate the excitation spectrum of a two-dimensional resonating valence bond (RVB) state. Treating the pi-flux phase with antiferromagnetic correlations as a variational ground state, we recover the long wavelength magnon as an "RVB exciton." However, this excitation does not exhaust the entire spectral weight and the high-energy spectrum is dominated by fermionic excitations. The latter can be observed directly by inelastic neutron scattering, and we predict their characteristic energy scales along different high symmetry directions in the magnetic Brillouin zone. We also interpret experimental results on two magnon Raman scattering and midinfrared absorption within this scenario.
我们研究了二维共振价键(RVB)态的激发光谱。将具有反铁磁关联的π-磁通相作为变分基态来处理,我们将长波长磁振子恢复为一个“RVB激子”。然而,这种激发并没有耗尽整个光谱权重,高能光谱由费米子激发主导。后者可以通过非弹性中子散射直接观测到,并且我们预测了它们在磁布里渊区沿不同高对称方向的特征能量尺度。我们还在此框架下解释了关于双磁振子拉曼散射和中红外吸收的实验结果。