Department of Earth Sciences, Durham University , Durham DH1 3LE, U.K.
Carbon Capture and Storage Programme, The Crown Estate , London W1S 2HX, U.K.
Environ Sci Technol. 2015 Nov 17;49(22):13510-8. doi: 10.1021/acs.est.5b02836. Epub 2015 Nov 4.
Injecting CO2 into deep saline formations represents an important component of many greenhouse-gas-reduction strategies for the future. A number of authors have posed concern over the thousands of injection wells likely to be needed. However, a more important criterion than the number of wells is whether the total cost of storing the CO2 is market-bearable. Previous studies have sought to determine the number of injection wells required to achieve a specified storage target. Here an alternative methodology is presented whereby we specify a maximum allowable cost (MAC) per ton of CO2 stored, a priori, and determine the corresponding potential operational storage capacity. The methodology takes advantage of an analytical solution for pressure build-up during CO2 injection into a cylindrical saline formation, accounting for two-phase flow, brine evaporation, and salt precipitation around the injection well. The methodology is applied to 375 saline formations from the U.K. Continental Shelf. Parameter uncertainty is propagated using Monte Carlo simulation with 10 000 realizations for each formation. The results show that MAC affects both the magnitude and spatial distribution of potential operational storage capacity on a national scale. Different storage prospects can appear more or less attractive depending on the MAC scenario considered. It is also shown that, under high well-injection rate scenarios with relatively low cost, there is adequate operational storage capacity for the equivalent of 40 years of U.K. CO2 emissions.
将二氧化碳注入深层盐水地层是未来许多减少温室气体策略的重要组成部分。许多作者对未来可能需要数千口注入井表示担忧。然而,比井的数量更重要的标准是储存二氧化碳的总成本是否可以承受市场压力。以前的研究试图确定实现特定储存目标所需的注入井数量。在这里,提出了一种替代方法,我们预先指定每吨储存二氧化碳的最大允许成本 (MAC),并确定相应的潜在运营储存能力。该方法利用了在圆柱形盐水地层中注入二氧化碳期间压力累积的解析解,考虑了两相流、盐水蒸发和注水井周围的盐沉淀。该方法应用于来自英国大陆架的 375 个盐水地层。使用 10,000 次蒙特卡罗模拟对每个地层的参数不确定性进行传播。结果表明,MAC 不仅影响潜在运营储存能力的大小,还影响其在全国范围内的空间分布。不同的存储前景可能根据考虑的 MAC 情景显得更有吸引力或吸引力较小。还表明,在成本相对较低的高井注入率情景下,有足够的运营储存能力来储存相当于英国 40 年的二氧化碳排放量。