Fang Huajing, Lin Ziyuan, Wang Xinsheng, Tang Chun-Yin, Chen Yan, Zhang Fan, Chai Yang, Li Qiang, Yan Qingfeng, Chan H L W, Dai Ji-Yan
Opt Express. 2015 Dec 14;23(25):31908-14. doi: 10.1364/OE.23.031908.
Molybdenum disulfide (MoS₂) as a promising 2D material has attracted extensive attentions due to its unique physical, optical and electrical properties. In this work, we demonstrate an infrared (IR) light gated MoS₂ transistor through a device composed of MoS₂ monolayer and a ferroelectric single crystal Pb(Mg(1/3)Nb(2/3))O₃-PbTiO₃ (PMN-PT). With a monolayer MoS₂ onto the top surface of (111) PMN-PT crystal, the drain current of MoS₂ channel can be modulated with infrared illumination and this modulation process is reversible. Thus, the transistor can work as a new kind of IR photodetector with a high IR responsivity of 114%/Wcm⁻². The IR response of MoS₂ transistor is attributed to the polarization change of PMN-PT single crystal induced by the pyroelectric effect which results in a field effect. Our result promises the application of MoS₂ 2D material in infrared optoelectronic devices. Combining with the intrinsic photocurrent feature of MoS₂ in the visible range, the MoS₂ on ferroelectric single crystal may be sensitive to a broadband wavelength of light.
二硫化钼(MoS₂)作为一种很有前景的二维材料,因其独特的物理、光学和电学性质而受到广泛关注。在这项工作中,我们通过由MoS₂单层和铁电单晶Pb(Mg(1/3)Nb(2/3))O₃-PbTiO₃(PMN-PT)组成的器件展示了一种红外(IR)光控MoS₂晶体管。在(111)PMN-PT晶体的顶表面上覆盖单层MoS₂,MoS₂沟道的漏极电流可以通过红外光照进行调制,并且这种调制过程是可逆的。因此,该晶体管可以作为一种新型的红外光电探测器工作,具有114%/Wcm⁻²的高红外响应率。MoS₂晶体管的红外响应归因于热释电效应引起的PMN-PT单晶的极化变化,这导致了场效应。我们的结果有望使MoS₂二维材料应用于红外光电器件。结合MoS₂在可见光范围内的固有光电流特性,铁电单晶上的MoS₂可能对宽带波长的光敏感。