Ortiz-Ambriz Antonio, Tierno Pietro
Department of Structure and Constituents of Matter, University of Barcelona, Avinguda Diagonal 647, 08028 Barcelona, Spain.
Institute of Nanoscience and Nanotechnology, IN2UB, Universitat de Barcelona, 08028 Barcelona, Spain.
Nat Commun. 2016 Feb 1;7:10575. doi: 10.1038/ncomms10575.
Artificial spin ice systems, namely lattices of interacting single domain ferromagnetic islands, have been used to date as microscopic models of frustration induced by lattice topology, allowing for the direct visualization of spin arrangements and textures. However, the engineering of frustrated ice states in which individual spins can be manipulated in situ and the real-time observation of their collective dynamics remain both challenging tasks. Inspired by recent theoretical advances, here we realize a colloidal version of an artificial spin ice system using interacting polarizable particles confined to lattices of bistable gravitational traps. We show quantitatively that ice-selection rules emerge in this frustrated soft matter system by tuning the strength of the pair interactions between the microscopic units. Via independent control of particle positioning and dipolar coupling, we introduce monopole-like defects and strings and use loops with defined chirality as an elementary unit to store binary information.
人工自旋冰系统,即相互作用的单畴铁磁岛晶格,迄今为止一直被用作由晶格拓扑结构引起的阻挫微观模型,从而能够直接观察自旋排列和纹理。然而,实现能够原位操纵单个自旋并实时观测其集体动力学的阻挫冰态仍是具有挑战性的任务。受近期理论进展的启发,我们在此利用局限于双稳重力阱晶格中的相互作用可极化粒子,实现了人工自旋冰系统的胶体版本。我们定量地表明,通过调节微观单元之间的成对相互作用强度,在这个阻挫软物质系统中会出现冰选择规则。通过对粒子位置和偶极耦合的独立控制,我们引入了类单极子缺陷和弦,并使用具有确定手性的环作为存储二进制信息的基本单元。