CNRS, Institut NÉEL, F-38000 Grenoble, France.
Université Grenoble Alpes, Institut NÉEL, F-38000 Grenoble, France.
Nature. 2016 Dec 15;540(7633):410-413. doi: 10.1038/nature20155. Epub 2016 Nov 28.
Artificial spin-ice systems are lithographically patterned arrangements of interacting magnetic nanostructures that were introduced as way of investigating the effects of geometric frustration in a controlled manner. This approach has enabled unconventional states of matter to be visualized directly in real space, and has triggered research at the frontier between nanomagnetism, statistical thermodynamics and condensed matter physics. Despite efforts to create an artificial realization of the square-ice model-a two-dimensional geometrically frustrated spin-ice system defined on a square lattice-no simple geometry based on arrays of nanomagnets has successfully captured the macroscopically degenerate ground-state manifold of the model. Instead, square lattices of nanomagnets are characterized by a magnetically ordered ground state that consists of local loop configurations with alternating chirality. Here we show that all of the characteristics of the square-ice model are observed in an artificial square-ice system that consists of two sublattices of nanomagnets that are vertically separated by a small distance. The spin configurations we image after demagnetizing our arrays reveal unambiguous signatures of a Coulomb phase and algebraic spin-spin correlations, which are characterized by the presence of 'pinch' points in the associated magnetic structure factor. Local excitations-the classical analogues of magnetic monopoles-are free to evolve in an extensively degenerate, divergence-free vacuum. We thus provide a protocol that could be used to investigate collective magnetic phenomena, including Coulomb phases and the physics of ice-like materials.
人工自旋冰系统是通过相互作用的磁性纳米结构的光刻图案排列而成的,其被引入是为了以受控的方式研究几何各向异性的影响。这种方法使得非常规物质的状态能够直接在实空间中可视化,并在纳米磁性、统计热力学和凝聚态物理的前沿引发了研究。尽管人们努力创造出一种对正方冰模型的人工实现——一个定义在正方形晶格上的二维几何各向异性自旋冰系统——但是没有任何简单的基于纳米磁铁阵列的几何形状成功地捕获了该模型的宏观简并基态。相反,纳米磁铁的正方形晶格的特征是具有交替手性的局部环配置的有序磁基态。在这里,我们表明,由两个垂直隔开一小段距离的纳米磁铁子晶格组成的人工正方冰系统中观察到了正方冰模型的所有特征。在我们对阵列退磁后,我们所成像的自旋构型揭示了库仑相和代数自旋-自旋相关性的明确特征,这表现在相关磁结构因子中存在“夹点”。局部激发——磁单极子的经典模拟物——可以在广泛简并、无散度的真空中自由演化。因此,我们提供了一种可以用来研究集体磁现象的方案,包括库仑相和冰状材料的物理。