Wang Yong-Lei, Ma Xiaoyu, Xu Jing, Xiao Zhi-Li, Snezhko Alexey, Divan Ralu, Ocola Leonidas E, Pearson John E, Janko Boldizsar, Kwok Wai-Kwong
Materials Science Division, Argonne National Laboratory, Argonne, IL, USA.
Department of Physics, University of Notre Dame, Notre Dame, IN, USA.
Nat Nanotechnol. 2018 Jul;13(7):560-565. doi: 10.1038/s41565-018-0162-7. Epub 2018 Jun 11.
Geometric frustration emerges when local interaction energies in an ordered lattice structure cannot be simultaneously minimized, resulting in a large number of degenerate states. The numerous degenerate configurations may lead to practical applications in microelectronics, such as data storage, memory and logic. However, it is difficult to achieve very high degeneracy, especially in a two-dimensional system. Here, we showcase in situ controllable geometric frustration with high degeneracy in a two-dimensional flux-quantum system. We create this in a superconducting thin film placed underneath a reconfigurable artificial-spin-ice structure. The tunable magnetic charges in the artificial-spin-ice strongly interact with the flux quanta in the superconductor, enabling switching between frustrated and crystallized flux quanta states. The different states have measurable effects on the superconducting critical current profile, which can be reconfigured by precise selection of the spin-ice magnetic state through the application of an external magnetic field. We demonstrate the applicability of these effects by realizing a reprogrammable flux quanta diode. The tailoring of the energy landscape of interacting 'particles' using artificial-spin-ices provides a new paradigm for the design of geometric frustration, which could illuminate a path to control new functionalities in other material systems, such as magnetic skyrmions, electrons and holes in two-dimensional materials, and topological insulators, as well as colloids in soft materials.
当有序晶格结构中的局部相互作用能无法同时达到最小时,就会出现几何阻挫,从而导致大量简并态。众多的简并构型可能会在微电子领域带来实际应用,比如数据存储、内存和逻辑。然而,很难实现非常高的简并度,尤其是在二维系统中。在此,我们展示了二维磁通量子系统中具有高简并度的原位可控几何阻挫。我们在置于可重构人工自旋冰结构下方的超导薄膜中实现了这一点。人工自旋冰中可调谐的磁荷与超导体中的磁通量子强烈相互作用,使得阻挫磁通量子态和结晶磁通量子态之间能够实现切换。不同的状态对超导临界电流分布有可测量的影响,通过施加外部磁场精确选择自旋冰磁态可以对其进行重新配置。我们通过实现一个可重新编程的磁通量子二极管来证明这些效应的适用性。利用人工自旋冰对相互作用“粒子”的能量景观进行剪裁,为几何阻挫的设计提供了一种新范式,这可能为控制其他材料系统中的新功能指明一条道路,这些材料系统包括磁性斯格明子、二维材料中的电子和空穴、拓扑绝缘体以及软材料中的胶体。