Schmidt Jürgen, Guggenmos Alexander, Hofstetter Michael, Chew Soo Hoon, Kleineberg Ulf
Opt Express. 2015 Dec 28;23(26):33564-78. doi: 10.1364/OE.23.033564.
High harmonic radiation is meanwhile nearly extensively used for the spectroscopic investigation of electron dynamics with ultimate time resolution. The majority of high harmonic beamlines provide linearly polarized radiation created in a gas target. However, circular polarization greatly extends the spectroscopic possibilities for high harmonics, especially in the analysis of samples with chirality or prominent spin polarization. We produced a free-standing multilayer foil as a transmission EUV quarter waveplate and applied it for the first time to high harmonic radiation. We measured a broadband (4.6 eV FWHM) ellipticity of 75% at 66 eV photon energy with a transmission efficiency of 5%. The helicity is switchable and the ellipticity can be adjusted to lower values by angle tuning. As a single element it can be easily integrated in any existing harmonic beamline without major changes.
与此同时,高谐波辐射几乎被广泛用于以极高的时间分辨率对电子动力学进行光谱研究。大多数高谐波光束线提供在气体靶中产生的线偏振辐射。然而,圆偏振极大地扩展了高谐波的光谱可能性,特别是在分析具有手性或显著自旋极化的样品时。我们制备了一种独立的多层箔作为透射式极紫外四分之一波片,并首次将其应用于高谐波辐射。我们在66 eV光子能量下测量到宽带(半高宽为4.6 eV)椭圆率为75%,传输效率为5%。螺旋度是可切换的,并且椭圆率可以通过角度调谐调整到更低的值。作为单个元件,它可以很容易地集成到任何现有的谐波光束线中,而无需进行重大更改。