Miller Owen D, Polimeridis Athanasios G, Homer Reid M T, Hsu Chia Wei, DeLacy Brendan G, Joannopoulos John D, Soljačić Marin, Johnson Steven G
Opt Express. 2016 Feb 22;24(4):3329-64. doi: 10.1364/OE.24.003329.
At visible and infrared frequencies, metals show tantalizing promise for strong subwavelength resonances, but material loss typically dampens the response. We derive fundamental limits to the optical response of absorptive systems, bounding the largest enhancements possible given intrinsic material losses. Through basic conservation-of-energy principles, we derive geometry-independent limits to per-volume absorption and scattering rates, and to local-density-of-states enhancements that represent the power radiated or expended by a dipole near a material body. We provide examples of structures that approach our absorption and scattering limits at any frequency; by contrast, we find that common "antenna" structures fall far short of our radiative LDOS bounds, suggesting the possibility for significant further improvement. Underlying the limits is a simple metric, |χ|2/Im χ for a material with susceptibility χ, that enables broad technological evaluation of lossy materials across optical frequencies.
在可见光和红外频率下,金属展现出了诱人的强亚波长共振前景,但材料损耗通常会削弱这种响应。我们推导了吸收性系统光学响应的基本极限,限定了在存在固有材料损耗的情况下可能实现的最大增强。通过基本的能量守恒原理,我们推导了与几何形状无关的每体积吸收和散射率的极限,以及局域态密度增强的极限,局域态密度增强表示材料体附近偶极子辐射或消耗的功率。我们给出了在任何频率下接近我们吸收和散射极限的结构示例;相比之下,我们发现常见的“天线”结构远远达不到我们的辐射局域态密度界限,这表明有显著进一步改进的可能性。这些极限的基础是一个简单的度量,即对于具有极化率χ的材料,|χ|²/Im χ,它能够对光学频率范围内的有损材料进行广泛的技术评估。