Wang Zhengzhi, Chiang Martin Y M
Biosystems and Biomaterials Division, National Institute of Standards and Technology (NIST), Gaithersburg, MD 20899, United States.
Biosystems and Biomaterials Division, National Institute of Standards and Technology (NIST), Gaithersburg, MD 20899, United States.
Dent Mater. 2016 Apr;32(4):551-60. doi: 10.1016/j.dental.2016.01.006. Epub 2016 Feb 23.
The effect of filler content in dental restorative composites on the polymerization shrinkage stress (PS) is not straightforward and has caused much debate in the literature. Our objective in this study was to clarify the PS/filler content relationship based on analytical and experimental approaches, so that guidelines for materials comparison in terms of PS and clinical selection of dental composites with various filler content can be provided.
Analytically, a simplified model based on linear elasticity was utilized to predict PS as a function of filler content under various compliances of the testing system, a cantilever beam-based instrument used in this study. The predictions were validated by measuring PS of composites synthesized using 50/50 mixtures of two common dimethacrylate resins with a variety of filler contents.
Both experiments and predictions indicated that the influence of filler content on the PS highly depended on the compliance of the testing system. Within the clinic-relevant range of compliances and for the specific sample configuration tested, the PS increased with increasing filler content at low compliance of instrument, while increasing the compliance caused the effect of filler content on the PS to gradually diminish. Eventually, at high compliance, the PS inverted and decreased with increasing filler content.
This compliance-dependent effect of filler content on PS suggests: (1) for materials comparison in terms of PS, the specific compliance at which the comparison being done should always be reported and (2) clinically, composites with relatively lower filler content could be selected for such cavities with relatively lower compliance (e.g. a Class-I cavity with thick tooth walls or the basal part in a cavity) and vice versa in order to reduce the final PS.
牙科修复复合材料中填料含量对聚合收缩应力(PS)的影响并非一目了然,在文献中引发了诸多争论。本研究的目的是基于分析和实验方法阐明PS与填料含量之间的关系,从而为根据PS进行材料比较以及临床选择不同填料含量的牙科复合材料提供指导。
在分析方面,利用基于线弹性的简化模型来预测PS作为填料含量的函数,该函数取决于本研究中使用的基于悬臂梁的测试系统的各种柔度。通过测量使用两种常见二甲基丙烯酸酯树脂的50/50混合物与各种填料含量合成的复合材料的PS来验证预测结果。
实验和预测均表明,填料含量对PS的影响高度依赖于测试系统的柔度。在临床相关的柔度范围内以及对于所测试的特定样品配置,在仪器柔度较低时,PS随填料含量的增加而增加,而增加柔度会使填料含量对PS的影响逐渐减弱。最终,在高柔度下,PS反转并随填料含量的增加而降低。
填料含量对PS的这种依赖于柔度的影响表明:(1)就PS而言进行材料比较时,应始终报告进行比较时的特定柔度;(2)在临床上,对于柔度相对较低的窝洞(例如牙壁较厚的I类洞或窝洞的基部),可以选择填料含量相对较低的复合材料,反之亦然,以降低最终的PS。