Mushenheim Peter C, Pendery Joel S, Weibel Douglas B, Spagnolie Saverio E, Abbott Nicholas L
Department of Chemical and Biological Engineering, University of Wisconsin-Madison, Madison, WI 53706;
Department of Biochemistry, University of Wisconsin-Madison, Madison, WI 53706;
Proc Natl Acad Sci U S A. 2016 May 17;113(20):5564-9. doi: 10.1073/pnas.1600836113. Epub 2016 May 2.
Liquid crystals (LCs), because of their long-range molecular ordering, are anisotropic, elastic fluids. Herein, we report that elastic stresses imparted by nematic LCs can dynamically shape soft colloids and tune their physical properties. Specifically, we use giant unilamellar vesicles (GUVs) as soft colloids and explore the interplay of mechanical strain when the GUVs are confined within aqueous chromonic LC phases. Accompanying thermal quenching from isotropic to LC phases, we observe the elasticity of the LC phases to transform initially spherical GUVs (diameters of 2-50 µm) into two distinct populations of GUVs with spindle-like shapes and aspect ratios as large as 10. Large GUVs are strained to a small extent (R/r < 1.54, where R and r are the major and minor radii, respectively), consistent with an LC elasticity-induced expansion of lipid membrane surface area of up to 3% and conservation of the internal GUV volume. Small GUVs, in contrast, form highly elongated spindles (1.54 < R/r < 10) that arise from an efflux of LCs from the GUVs during the shape transformation, consistent with LC-induced straining of the membrane leading to transient membrane pore formation. A thermodynamic analysis of both populations of GUVs reveals that the final shapes adopted by these soft colloids are dominated by a competition between the LC elasticity and an energy (∼0.01 mN/m) associated with the GUV-LC interface. Overall, these results provide insight into the coupling of strain in soft materials and suggest previously unidentified designs of LC-based responsive and reconfigurable materials.
液晶(LCs)由于其长程分子有序性,是各向异性的弹性流体。在此,我们报告向列型液晶施加的弹性应力可动态塑造软胶体并调节其物理性质。具体而言,我们使用巨型单层囊泡(GUVs)作为软胶体,并探究当GUVs被限制在水性发色液晶相内时的机械应变相互作用。随着从各向同性相到液晶相的热猝灭,我们观察到液晶相的弹性将最初呈球形的GUVs(直径为2 - 50 µm)转变为两个不同群体的具有纺锤状形状且纵横比高达10的GUVs。大的GUVs受到的应变较小(R/r < 1.54,其中R和r分别为长半径和短半径),这与液晶弹性导致脂质膜表面积增加高达3%且GUV内部体积守恒相一致。相比之下,小的GUVs形成高度拉长的纺锤体(1.54 < R/r < 10),这是由于在形状转变过程中液晶从GUVs流出所致,与液晶诱导的膜应变导致瞬时膜孔形成相一致。对这两个群体的GUVs进行的热力学分析表明,这些软胶体最终采用的形状主要由液晶弹性与与GUV - 液晶界面相关的能量(约0.01 mN/m)之间的竞争决定。总体而言,这些结果深入了解了软材料中应变的耦合,并提出了基于液晶的响应性和可重构材料以前未被识别的设计。