Zheng Yan-Zong, Soo Yun-Liang, Chang Shih-Lin
Department of Physics, National Tsing Hua University, 101, Section 2, Kuang Fu Road, Hsinchu, Taiwan 30013.
National Synchrotron Radiation Research Center, 101, Hsin-Ann Road, Hsinchu Science Park, Hsinchu, Taiwan 30076.
Sci Rep. 2016 May 9;6:25580. doi: 10.1038/srep25580.
Interfacial strains are important factors affecting the structural and physical properties of crystalline multilayers and heterojunctions, and the performance of the devices made of multilayers used, for example, in nanowires, optoelectronic components, and many other applications. Currently existing strain measurement methods, such as grazing incidence X-ray diffraction (GIXD), cross-section transmission electron microscope, TEM, and coherent diffractive imaging, CDI, are limited by either the nanometer spatial resolution, penetration depth, or a destructive nature. Here we report a new non-destructive method of direct mapping the interfacial strain of [001] Si0.7Ge0.3/Si along the depth up to ~287 nm below the interface using three-beam Bragg-surface X-ray diffraction (BSD), where one wide-angle symmetric Bragg reflection and a surface reflection are simultaneously involved. Our method combining with the dynamical diffraction theory simulation can uniquely provide unit cell dimensions layer by layer, and is applicable to thicker samples.
界面应变是影响晶体多层膜和异质结的结构与物理性质,以及由多层膜制成的器件性能的重要因素,这些多层膜用于例如纳米线、光电器件及许多其他应用中。目前现有的应变测量方法,如掠入射X射线衍射(GIXD)、截面透射电子显微镜(TEM)和相干衍射成像(CDI),受到纳米级空间分辨率、穿透深度或破坏性的限制。在此,我们报告了一种新的无损方法,利用三束布拉格表面X射线衍射(BSD)沿着界面以下高达约287 nm的深度直接绘制[001] Si0.7Ge0.3/Si的界面应变,其中同时涉及一个广角对称布拉格反射和一个表面反射。我们的方法与动态衍射理论模拟相结合,可以逐层唯一地提供晶胞尺寸,并且适用于更厚的样品。