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大块陨石及其内含物中的钨同位素——对太阳原行星盘中前太阳成分加工的启示

Tungsten isotopes in bulk meteorites and their inclusions-Implications for processing of presolar components in the solar protoplanetary disk.

作者信息

Holst J C, Paton C, Wielandt D, Bizzarro M

机构信息

Centre for Star and Planet Formation and Natural History Museum of Denmark, University of Copenhagen, DK-1350 Copenhagen, Denmark.

出版信息

Meteorit Planet Sci. 2015 Sep 3;50(9):1643-1660. doi: 10.1111/maps.12488.

Abstract

We present high precision, low- and high-resolution tungsten isotope measurements of iron meteorites Cape York (IIIAB), Rhine Villa (IIIE), Bendego (IC), and the IVB iron meteorites Tlacotepec, Skookum, and Weaver Mountains, as well as CI chondrite Ivuna, a CV3 chondrite refractory inclusion (CAI BE), and terrestrial standards. Our high precision tungsten isotope data show that the distribution of the rare -process nuclide W is homogeneous among chondrites, iron meteorites, and the refractory inclusion. One exception to this pattern is the IVB iron meteorite group, which displays variable excesses relative to the terrestrial standard, possibly related to decay of rare Os. Such anomalies are not the result of analytical artifacts and cannot be caused by sampling of a protoplanetary disk characterized by -process isotope heterogeneity. In contrast, we find that W is variable due to a nucleosynthetic -process deficit/-process excess among chondrites and iron meteorites. This variability supports the widespread nucleosynthetic /-process heterogeneity in the protoplanetary disk inferred from other isotope systems and we show that W and Ni isotope variability is correlated. Correlated isotope heterogeneity for elements of distinct nucleosynthetic origin (W and Ni) is best explained by thermal processing in the protoplanetary disk during which thermally labile carrier phases are unmixed by vaporization thereby imparting isotope anomalies on the residual processed reservoir.

摘要

我们展示了对铁陨石约克角(IIIAB)、莱茵别墅(IIIE)、本迪戈(IC)以及IVB铁陨石特拉科特佩克、斯库库姆和韦弗山的高精度、低分辨率和高分辨率钨同位素测量结果,以及CI球粒陨石伊武纳、CV3球粒陨石难熔包体(CAI BE)和地球标准物质的测量结果。我们的高精度钨同位素数据表明,稀有过程核素钨在球粒陨石、铁陨石和难熔包体中的分布是均匀的。这种模式的一个例外是IVB铁陨石群,相对于地球标准物质,它显示出可变的过剩,这可能与稀有锇的衰变有关。这种异常不是分析假象的结果,也不可能是由具有过程同位素异质性的原行星盘采样引起的。相反,我们发现,由于球粒陨石和铁陨石中核合成过程亏损/过程过剩,钨是可变的。这种变异性支持了从其他同位素系统推断出的原行星盘中广泛存在的核合成/过程异质性,并且我们表明钨和镍同位素变异性是相关的。不同核合成起源元素(钨和镍)的相关同位素异质性最好用原行星盘中的热过程来解释,在此过程中,热不稳定载体相通过汽化而分离,从而在残余的加工储库中产生同位素异常。

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