使用负载型金催化剂通过CO加氢直接合成乙醇。
Direct synthesis of ethanol via CO hydrogenation using supported gold catalysts.
作者信息
Wang Dong, Bi Qingyuan, Yin Guoheng, Zhao Wenli, Huang Fuqiang, Xie Xiaoming, Jiang Mianheng
机构信息
State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, P. R. China and State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, P. R. China.
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, P. R. China.
出版信息
Chem Commun (Camb). 2016 Dec 6;52(99):14226-14229. doi: 10.1039/c6cc08161d.
An efficient titania supported Au nanocluster (NC) has been prepared for the direct synthesis of useful EtOH from CO and H. The unique creation of an excellent synergistic effect between Au NCs and the underlying TiO support, especially the anatase crystal phase with abundant oxygen vacancies, can achieve the high performance for EtOH synthesis under moderate and practical conditions.
已经制备了一种高效的二氧化钛负载金纳米团簇（NC），用于从一氧化碳和氢气直接合成有用的乙醇。金纳米团簇与底层二氧化钛载体之间独特地产生了优异的协同效应，特别是具有大量氧空位的锐钛矿晶相，能够在温和且实际可行的条件下实现乙醇合成的高性能。
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