Zakharko Yuriy, Held Martin, Graf Arko, Rödlmeier Tobias, Eckstein Ralph, Hernandez-Sosa Gerardo, Hähnlein Bernd, Pezoldt Jörg, Zaumseil Jana
Institute for Physical Chemistry, Universität Heidelberg , D-69120 Heidelberg, Germany.
Light Technology Institute, Karlsruhe Institute of Technology, D-76131 Karlsruhe, Germany; InnovationLab, Speyerer Straße 4, D-69115 Heidelberg, Germany.
ACS Photonics. 2016 Dec 21;3(12):2225-2230. doi: 10.1021/acsphotonics.6b00491. Epub 2016 Nov 9.
Hybrid photonic-plasmonic modes in periodic arrays of metallic nanostructures offer a promising trade-off between high-quality cavities and subdiffraction mode confinement. However, their application in electrically driven light-emitting devices is hindered by their sensitivity to the surrounding environment and to charge injecting metallic electrodes in particular. Here, we demonstrate that the planar structure of light-emitting field-effect transistor (LEFET) ensures undisturbed operation of the characteristic modes. We incorporate a square array of gold nanodisks into the charge transporting and emissive layer of a polymer LEFET in order to tailor directionality and emission efficiency via the Purcell effect and variation of the fractional local density of states in particular. Angle- and polarization-resolved spectra confirm that the enhanced electroluminescence correlates with the dispersion curves of the surface lattice resonances supported by these structures. These LEFETs reach current densities on the order of 10 kA/cm, which may pave the way toward practical optoelectronic devices with tailored emission patterns and potentially electrically pumped plasmonic lasers.
金属纳米结构周期性阵列中的混合光子 - 等离子体模式在高质量腔和亚衍射模式限制之间提供了一种很有前景的权衡。然而,它们在电驱动发光器件中的应用受到其对周围环境特别是对注入电荷的金属电极的敏感性的阻碍。在这里,我们证明发光场效应晶体管(LEFET)的平面结构确保了特征模式的不受干扰的运行。我们将金纳米盘的方形阵列并入聚合物LEFET的电荷传输和发射层中,以便特别是通过珀塞尔效应和分数局部态密度的变化来调整方向性和发射效率。角度和偏振分辨光谱证实,增强的电致发光与这些结构所支持的表面晶格共振的色散曲线相关。这些LEFET达到了10 kA/cm量级的电流密度,这可能为具有定制发射模式和潜在电泵浦等离子体激光器功能的实用光电器件铺平道路。