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发光双曲超表面。

Luminescent hyperbolic metasurfaces.

机构信息

Department of Electrical and Computer Engineering, University of California, San Diego, 9500 Gilman Drive, Mail code 0407, La Jolla, California 92093, USA.

Material Science and Engineering Program, University of California, San Diego, La Jolla, California, 92093, USA.

出版信息

Nat Commun. 2017 Jan 9;8:13793. doi: 10.1038/ncomms13793.

Abstract

When engineered on scales much smaller than the operating wavelength, metal-semiconductor nanostructures exhibit properties unobtainable in nature. Namely, a uniaxial optical metamaterial described by a hyperbolic dispersion relation can simultaneously behave as a reflective metal and an absorptive or emissive semiconductor for electromagnetic waves with orthogonal linear polarization states. Using an unconventional multilayer architecture, we demonstrate luminescent hyperbolic metasurfaces, wherein distributed semiconducting quantum wells display extreme absorption and emission polarization anisotropy. Through normally incident micro-photoluminescence measurements, we observe absorption anisotropies greater than a factor of 10 and degree-of-linear polarization of emission >0.9. We observe the modification of emission spectra and, by incorporating wavelength-scale gratings, show a controlled reduction of polarization anisotropy. We verify hyperbolic dispersion with numerical simulations that model the metasurface as a composite nanoscale structure and according to the effective medium approximation. Finally, we experimentally demonstrate >350% emission intensity enhancement relative to the bare semiconducting quantum wells.

摘要

当工程规模远小于工作波长时,金属-半导体纳米结构表现出自然界中无法获得的性质。具体来说,具有双曲色散关系的单轴光超材料可以同时表现为对具有正交线性偏振态的电磁波的反射金属和吸收或发射半导体。我们使用一种非传统的多层架构,展示了发光的双曲超表面,其中分布式半导体量子阱显示出极端的吸收和发射偏振各向异性。通过正常入射微光致发光测量,我们观察到吸收各向异性大于 10 倍,发射的线偏振度>0.9。我们观察到发射光谱的修饰,并通过结合波长尺度的光栅,显示出对偏振各向异性的控制减小。我们通过数值模拟验证了超材料的双曲色散,该模拟将超表面建模为复合纳米结构,并根据有效媒质近似。最后,我们实验证明与裸半导体量子阱相比,发射强度增强了超过 350%。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b79e/5473634/366ec721e397/ncomms13793-f1.jpg

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