Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Str. 40, D-01187 Dresden, Germany.
Leibniz Institut für Festkörper- und Werkstoffforschung IFW Dresden, D-01171 Dresden, Germany.
Nat Commun. 2017 Jan 9;8:13942. doi: 10.1038/ncomms13942.
The rare-earth monopnictide LaBi exhibits exotic magneto-transport properties, including an extremely large and anisotropic magnetoresistance. Experimental evidence for topological surface states is still missing although band inversions have been postulated to induce a topological phase in LaBi. In this work, we have revealed the existence of surface states of LaBi through the observation of three Dirac cones: two coexist at the corners and one appears at the centre of the Brillouin zone, by employing angle-resolved photoemission spectroscopy in conjunction with ab initio calculations. The odd number of surface Dirac cones is a direct consequence of the odd number of band inversions in the bulk band structure, thereby proving that LaBi is a topological, compensated semimetal, which is equivalent to a time-reversal invariant topological insulator. Our findings provide insight into the topological surface states of LaBi's semi-metallicity and related magneto-transport properties.
稀土单磷化物 LaBi 表现出奇异的磁输运性质,包括极其大且各向异性的磁阻。尽管已经假设能带反转会在 LaBi 中诱导拓扑相,但实验证据仍缺失拓扑表面态。在这项工作中,我们通过角分辨光发射光谱学结合第一性原理计算,观察到了三个狄拉克锥,证明了 LaBi 表面态的存在:两个位于顶角共存,一个出现在布里渊区中心。这种情况是由于体带结构中的带反转数量为奇数,从而证明了 LaBi 是拓扑补偿半金属,相当于时间反演不变的拓扑绝缘体。我们的发现为 LaBi 的半金属性和相关磁输运性质的拓扑表面态提供了深入的了解。