Liu Z K, Yang L X, Wu S-C, Shekhar C, Jiang J, Yang H F, Zhang Y, Mo S-K, Hussain Z, Yan B, Felser C, Chen Y L
School of Physical Science and Technology, ShanghaiTech University and CAS-Shanghai Science Research Center, Shanghai 201203, China.
State Key Laboratory of Low Dimensional Quantum Physics, Department of Physics and Collaborative Innovation Center for Quantum Matter, Tsinghua University, Beijing 100084, China.
Nat Commun. 2016 Sep 27;7:12924. doi: 10.1038/ncomms12924.
Topological quantum materials represent a new class of matter with both exotic physical phenomena and novel application potentials. Many Heusler compounds, which exhibit rich emergent properties such as unusual magnetism, superconductivity and heavy fermion behaviour, have been predicted to host non-trivial topological electronic structures. The coexistence of topological order and other unusual properties makes Heusler materials ideal platform to search for new topological quantum phases (such as quantum anomalous Hall insulator and topological superconductor). By carrying out angle-resolved photoemission spectroscopy and ab initio calculations on rare-earth half-Heusler compounds LnPtBi (Ln=Lu, Y), we directly observe the unusual topological surface states on these materials, establishing them as first members with non-trivial topological electronic structure in this class of materials. Moreover, as LnPtBi compounds are non-centrosymmetric superconductors, our discovery further highlights them as promising candidates of topological superconductors.
拓扑量子材料代表了一类具有奇异物理现象和新颖应用潜力的新型物质。许多具有丰富涌现性质(如异常磁性、超导性和重费米子行为)的赫斯勒化合物,已被预测具有非平凡的拓扑电子结构。拓扑序与其他异常性质的共存,使赫斯勒材料成为寻找新拓扑量子相(如量子反常霍尔绝缘体和拓扑超导体)的理想平台。通过对稀土半赫斯勒化合物LnPtBi(Ln = Lu、Y)进行角分辨光电子能谱和从头算计算,我们直接观察到这些材料上不寻常的拓扑表面态,将它们确立为这类材料中具有非平凡拓扑电子结构的首批成员。此外,由于LnPtBi化合物是非中心对称超导体,我们的发现进一步突出了它们作为拓扑超导体的有前景的候选者。