Pescaglini Andrea, Biswas Subhajit, Cammi Davide, Ronning Carsten, Holmes Justin D, Iacopino Daniela
Tyndall National Institute, Dyke Parade, Cork, Ireland.
Phys Chem Chem Phys. 2017 May 31;19(21):14042-14047. doi: 10.1039/c7cp01356f.
Nanoscale heating production using nanowires has been shown to be particularly attractive for a number of applications including nanostructure growth, localized doping, transparent heating and sensing. However, all proof-of-concept devices proposed so far relied on the use of highly conductive nanomaterials, typically metals or highly doped semiconductors. In this article, we demonstrate a novel nanoheater architecture based on a single semiconductor nanowire field-effect transistor (NW-FET). Nominally undoped ZnO nanowires were incorporated into three-terminal devices whereby control of the nanowire temperature at a given source-drain bias was achieved by additional charge carriers capacitatively induced via the third gate electrode. Joule-heating selective ablation of poly(methyl methacrylate) deposited on ZnO nanowires was shown, demonstrating the ability of the proposed NW-FET configuration to enhance by more than one order of magnitude the temperature of a ZnO nanowire, compared to traditional two-terminal configurations. These findings demonstrate the potential of field-effect architectures to improve Joule heating power in nanowires, thus vastly expanding the range of suitable materials and applications for nanowire-based nanoheaters.
利用纳米线产生纳米级热量已被证明在包括纳米结构生长、局部掺杂、透明加热和传感在内的许多应用中具有特别的吸引力。然而,迄今为止提出的所有概念验证器件都依赖于使用高导电性的纳米材料,通常是金属或高掺杂半导体。在本文中,我们展示了一种基于单一半导体纳米线场效应晶体管(NW-FET)的新型纳米加热器架构。将名义上未掺杂的ZnO纳米线集成到三端器件中,通过经由第三栅电极电容性感应的额外电荷载流子,实现了在给定源漏偏压下对纳米线温度的控制。展示了沉积在ZnO纳米线上的聚甲基丙烯酸甲酯的焦耳热选择性烧蚀,这表明与传统的两端配置相比,所提出的NW-FET配置能够将ZnO纳米线的温度提高一个多数量级。这些发现证明了场效应架构在提高纳米线中焦耳热功率方面的潜力,从而极大地扩展了基于纳米线的纳米加热器的适用材料和应用范围。