Department of Nuclear Physics, Research School of Physics and Engineering, Australian National University, Canberra, ACT 2601, Australia.
Department of Nuclear Physics, Research School of Physics and Engineering, Australian National University, Canberra, ACT 2601, Australia.
J Environ Radioact. 2017 Nov;178-179:349-353. doi: 10.1016/j.jenvrad.2017.05.009. Epub 2017 May 16.
A slice from a Porites Lutea coral core collected inside the Enewetak Atoll lagoon, within 15 km of all major nuclear tests conducted at the atoll, was analysed for U, Pu and Pu over the time interval 1952-1964 using a higher time resolution than previously reported for a parallel slice from the same core. In addition two sediment samples from the Koa and Oak craters were analysed. The strong peaks in the concentrations of U and Pu in the testing years are confirmed to be considerably wider than the flushing time of the lagoon. This is likely due to the growth mechanism of the coral. Following the last test in 1958 atom concentrations of both U and Pu decreased from their peak values by more than 95% and showed a seasonal signal thereafter. Between 1959 and 1964 the weighted average of the Pu/Pu atom ratio is 0.124 ± 0.008 which is similar to that in the lagoon sediments (0.129 ± 0.006) but quite distinct from the global fallout value of ∼0.18. This, and the high Pu and U concentrations in the sediments, provides clear evidence that the post-testing signal in the coral is dominated by remobilisation of the isotopes from the lagoon sediments rather than from global fallout.
从埃尼威托克环礁泻湖内采集的一枚多孔鹿角珊瑚岩芯的切片进行了分析,该岩芯位于距离环礁所有主要核试验地点 15 公里以内,分析了 1952 年至 1964 年间 U、Pu 和 Pu 的浓度,时间分辨率高于之前对同一岩芯的平行切片的报道。此外,还分析了来自 Koa 和 Oak 火山口的两个沉积物样本。在试验年份中,U 和 Pu 浓度的强烈峰值被证实比泻湖的冲洗时间宽得多。这可能是由于珊瑚的生长机制。自 1958 年最后一次试验以来,U 和 Pu 的原子浓度均从峰值下降了 95%以上,并在此后显示出季节性信号。1959 年至 1964 年间,Pu/Pu 原子比的加权平均值为 0.124±0.008,与泻湖沉积物中的值(0.129±0.006)相似,但与全球沉降值(约 0.18)明显不同。这一点,以及沉积物中高浓度的 Pu 和 U,提供了明确的证据,表明珊瑚中的试验后信号主要是由泻湖沉积物中的同位素再迁移引起的,而不是由全球沉降引起的。