Institute of the Environment and Sustainability, University of California , Los Angeles, California 90095, United States.
Department of Environmental Health Sciences, Jonathan and Karin Fielding School of Public Health, University of California , Los Angeles, California 90095, United States.
Environ Sci Technol. 2017 Jun 20;51(12):6990-6998. doi: 10.1021/acs.est.6b06464. Epub 2017 Jun 2.
Particle emissions from heavy-duty vehicles (HDVs) have significant environmental and public health impacts. This study measured total particle number emission factors (PNEFs) from six newly certified HDVs powered by diesel and compressed natural gas totaling over 6800 miles of on-road operation in California. Distance-, fuel- and work-based PNEFs were calculated for each vehicle. Distance-based PNEFs of vehicles equipped with original equipment manufacturer (OEM) diesel particulate filters (DPFs) in this study have decreased by 355-3200 times compared to a previous retrofit DPF dynamometer study. Fuel-based PNEFs were consistent with previous studies measuring plume exhaust in the ambient air. Meanwhile, on-road PNEF shows route and technology dependence. For vehicles with OEM DPFs and Selective Catalytic Reduction Systems, PNEFs under highway driving (i.e., 3.34 × 10 to 2.29 × 10 particles/mile) were larger than those measured on urban and drayage routes (i.e., 5.06 × 10 to 1.31 × 10 particles/mile). This is likely because a significant amount of nucleation mode volatile particles were formed when the DPF outlet temperature reached a critical value, usually over 310 °C, which was commonly achieved when vehicle speed sustained over 45 mph. A model year 2013 diesel HDV produced approximately 10 times higher PNEFs during DPF active regeneration events than nonactive regeneration.
重型车辆(HDV)的颗粒物排放对环境和公共健康有重大影响。本研究测量了六辆新认证的 HDV 的总颗粒物数排放因子(PNEF),这些车辆在加利福尼亚州进行了超过 6800 英里的道路行驶,使用的燃料为柴油和压缩天然气。为每辆车计算了基于距离、燃料和工作的 PNEF。与之前的 retrofit DPF 测功机研究相比,本研究中配备原始设备制造商(OEM)柴油颗粒过滤器(DPF)的车辆的基于距离的 PNEF 减少了 355 至 3200 倍。基于燃料的 PNEF 与之前在环境空气中测量羽流废气的研究一致。同时,道路 PNEF 显示出路线和技术的依赖性。对于配备 OEM DPF 和选择性催化还原系统的车辆,在高速公路行驶下(即 3.34×10 至 2.29×10 个颗粒/英里)的 PNEF 大于在城市和拖运路线下测量的 PNEF(即 5.06×10 至 1.31×10 个颗粒/英里)。这可能是因为当 DPF 出口温度达到临界值(通常超过 310°C)时,大量的成核模式挥发性颗粒形成,这通常是在车速持续超过 45 英里/小时时实现的。一辆 2013 年的柴油 HDV 在 DPF 主动再生期间产生的 PNEF 比非主动再生期间高约 10 倍。