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社会经济和气象因素对水库空气质量的影响:以中国重庆三峡水库(TGRC)为例的十年研究

Impact of socioeconomic and meteorological factors on reservoirs' air quality: a case in the Three Gorges Reservoir of Chongqing (TGRC), China over a 10-year period.

作者信息

Peng Ying, Zhou Fengwu, Cui Jian, Du Ke, Leng Qiangmei, Yang Fumo, Chan Andy, Zhao Hongting

机构信息

Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing, 210008, China.

University of Chinese Academy of Sciences, Beijing, 100049, China.

出版信息

Environ Sci Pollut Res Int. 2017 Jul;24(19):16206-16219. doi: 10.1007/s11356-017-9221-0. Epub 2017 May 24.

Abstract

The Three Gorges Dam's construction and industrial transfer have resulted in a new air pollution pattern with the potential to threaten the reservoir eco-environment. To assess the impact of socioeconomic factors on the pattern of air quality vairation and economical risks, concentrations of SO, NO, and PM, industry genres, and meteorological conditions were selected in the Three Gorges Reservoir of Chongqing (TGRC) during 2006-2015. Results showed that air quality had improved to some extent, but atmospheric NO showed an increased trend during 2011-2015. Spatially, higher atmospheric NO extended to the surrounding area. The primary industry, especially for agriculture, had shown to be responsible for the remarkable increase of atmospheric NO (p < 0.01) due to the direct burning of agricultural straws and the emission of livestock breeding. The improvement of regional industrial structure and industrialization benefited air pollutant reductions, but construction industries had inhibited the improvement of regional air quality. In the tertiary industry, the cargo industry at ports had significantly decreased atmospheric NO as a result of eliminating the obsoleted small ships. Contrarily, the highway transportation had brought more air pollutants. The relative humidity was shown to be the main meteorological factor, which had an extremely remarkable relation with atmospheric SO (p < 0.01) and a significant correlation with atmospheric NO (p < 0.05), respectively. In the future, the development of agriculture and livestock breeding would make regional air quality improvement difficult, and atmospheric SO, NO, and PM deposition would aggravate regional soil and water acidification and reactivate heavy metal in soil and sediment, further to pose a high level of ecological risk in the TGRC and other countries with reservoirs in the world.

摘要

三峡大坝的建设和产业转移导致了一种新的空气污染模式,有可能威胁水库生态环境。为评估社会经济因素对空气质量变化模式和经济风险的影响,选取了2006 - 2015年重庆三峡水库(TGRC)的SO、NO和PM浓度、产业类型及气象条件。结果表明,空气质量有一定程度改善,但2011 - 2015年大气NO呈上升趋势。在空间上,较高的大气NO浓度扩展到了周边地区。第一产业,尤其是农业,由于农作物秸秆直接燃烧和畜禽养殖排放,已被证明是大气NO显著增加的原因(p < 0.01)。区域产业结构的改善和工业化有利于空气污染物减排,但建筑业抑制了区域空气质量的改善。在第三产业中,港口货运业因淘汰老旧小船显著降低了大气NO浓度。相反,公路运输带来了更多空气污染物。相对湿度被证明是主要气象因素,它与大气SO分别具有极显著关系(p < 0.01),与大气NO具有显著相关性(p < 0.05)。未来,农业和畜禽养殖的发展将使区域空气质量改善变得困难,大气SO、NO和PM沉降将加剧区域土壤和水体酸化,并使土壤和沉积物中的重金属活化,进而在TGRC及世界其他有水库的国家造成高水平的生态风险。

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