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中国北京燃气燃烧产生的有害空气污染物(HAPs)的历史和未来排放。

Historical and future emission of hazardous air pollutants (HAPs) from gas-fired combustion in Beijing, China.

机构信息

National Engineering Research Center of Urban Environmental Pollution Control, Beijing Municipal Research Institute of Environmental Protection, Beijing, 100037, China.

State Key Joint Laboratory of Environmental Simulation & Pollution Control, School of Environment, Beijing Normal University, Beijing, 100875, China.

出版信息

Environ Sci Pollut Res Int. 2017 Jul;24(20):16946-16957. doi: 10.1007/s11356-017-9260-6. Epub 2017 Jun 3.

Abstract

The consumption of natural gas in Beijing has increased in the past decade due to energy structure adjustments and air pollution abatement. In this study, an integrated emission inventory of hazardous air pollutants (HAPs) emitted from gas-fired combustion in Beijing was developed for the period from 2000 to 2014 using a technology-based approach. Future emission trends were projected through 2030 based on current energy-related and emission control policies. We found that emissions of primary HAPs exhibited an increasing trend with the rapid increase in natural gas consumption. Our estimates indicated that the total emissions of NO , particulate matter (PM), PM, CO, VOCs, SO, black carbon, Pb, Cd, Hg, As, Cr, Cu, Ni, Zn, polychlorinated dibenzo-p-dioxins and dibenzofurans, and benzo[a]pyrene from gas-fired combustion in Beijing were approximately 22,422 t, 1042 t, 781 t, 19,097 t, 653 t, 82 t, 19 t, 0.6 kg, 0.1 kg, 43 kg, 52 kg, 0.3 kg, 0.03 kg, 4.3 kg, 0.6 kg, 216 μg, and 242 g, respectively, in 2014. To mitigate the associated air pollution and health risks caused by gas-fired combustion, stricter emission standards must be established. Additionally, combustion optimization and flue gas purification system could be used for lowering NO emissions from gas-fired combustion, and gas-fired facilities should be continuously monitored based on emission limits. Graphical abstract Spatial distribution and typical live photos of gas-fired boiler in Beijing.

摘要

由于能源结构调整和空气污染治理,北京的天然气消费量在过去十年中有所增加。本研究采用基于技术的方法,针对 2000 年至 2014 年期间,开发了一个综合排放清单,以估算燃气燃烧排放的有害空气污染物(HAPs)。根据当前的能源相关和排放控制政策,预测了 2030 年的未来排放趋势。我们发现,随着天然气消费的快速增长,主要 HAPs 的排放量呈上升趋势。我们的估算表明,北京燃气燃烧产生的总排放量约为 22422 吨,其中氮氧化物(NOx)、颗粒物(PM)、细颗粒物(PM2.5)、一氧化碳(CO)、挥发性有机化合物(VOCs)、二氧化硫(SO2)、黑碳、铅(Pb)、镉(Cd)、汞(Hg)、砷(As)、铬(Cr)、铜(Cu)、镍(Ni)、锌(Zn)、多氯二苯并对二恶英和多氯二苯并呋喃(PCDD/Fs)以及苯并[a]芘分别为 22422 吨、1042 吨、781 吨、19097 吨、653 吨、82 吨、19 吨、0.6 千克、0.1 千克、43 千克、52 千克、0.3 千克、0.03 千克、4.3 千克、0.6 千克、216 微克和 242 克。为了减轻燃气燃烧造成的空气污染和健康风险,必须制定更严格的排放标准。此外,可以采用燃烧优化和烟气净化系统来降低燃气燃烧产生的氮氧化物排放,并且应根据排放限值对燃气设施进行持续监测。

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