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剪切屈服应力流体中的非平凡流变指数。

Non-trivial rheological exponents in sheared yield stress fluids.

机构信息

Laboratoire de Physique Théorique, ENS & PSL University, UPMC & Sorbonne Universités, F-75005 Paris, France.

Université Grenoble Alpes, LIPHY, F-38000 Grenoble, France and CNRS, LIPHY, F-38000 Grenoble, France.

出版信息

Soft Matter. 2017 Jul 14;13(26):4653-4660. doi: 10.1039/c6sm02702d. Epub 2017 Jun 15.

Abstract

In this work we discuss possible physical origins of non-trivial exponents in the athermal rheology of soft materials at low but finite driving rates. A key ingredient in our scenario is the presence of a self-consistent mechanical noise that stems from the spatial superposition of long-range elastic responses to localized plastically deforming regions. We study analytically a mean-field model, in which this mechanical noise is accounted for by a stress diffusion term coupled to the plastic activity. Within this description we show how a dependence of the shear modulus and/or the local relaxation time on the shear rate introduces corrections to the usual mean-field prediction, concerning the Herschel-Bulkley-type rheological response of exponent 1/2. This feature of the mean-field picture is then shown to be robust with respect to structural disorder and partial relaxation of the local stress. We test this prediction numerically on a mesoscopic lattice model that implements explicitly the long-range elastic response to localized shear transformations, and we conclude on how our scenario might be tested in rheological experiments.

摘要

在这项工作中,我们讨论了在低但有限驱动速率下软物质非平凡无热流变学中可能的物理起源。我们方案中的一个关键要素是存在自洽的机械噪声,它源于对局部塑性变形区域的长程弹性响应的空间叠加。我们分析了一个平均场模型,其中这种机械噪声通过与塑性活动耦合的应力扩散项来表示。在这种描述中,我们展示了剪切模量和/或局部松弛时间对剪切率的依赖性如何对通常的平均场预测进行修正,涉及到赫谢尔-布尔克利型流变学响应的 1/2 指数。然后,我们通过显式实现局部剪切变形的长程弹性响应的介观格点模型对平均场图像的这一特征进行了数值测试,并得出了我们的方案如何在流变学实验中进行测试的结论。

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