Vasisht Vishwas V, Chaudhuri Pinaki, Martens Kirsten
Department of Physics, Indian Institute of Technology, Palakkad 678557, India.
Univ. Grenoble Alpes, CNRS, LIPhy, 38000 Grenoble, France.
Soft Matter. 2022 Aug 31;18(34):6426-6436. doi: 10.1039/d2sm00615d.
In soft amorphous materials, shear cessation after large shear deformation leads to configurations having residual shear stress. The origin of these states and the distribution of the local shear stresses within the material is not well understood, despite its importance for the change in material properties and consequent applications. In this work, we use molecular dynamics simulations of a model dense non-Brownian soft amorphous material to probe the non-trivial relaxation process towards a residual stress state. We find that, similar to thermal glasses, an increase in shear rate prior to the shear cessation leads to lower residual stress states. We rationalise our findings using a mesoscopic elasto-plastic description that explicitly includes a long range elastic response to local shear transformations. We find that after flow cessation the initial stress relaxation indeed depends on the pre-sheared stress state, but the final residual stress is majorly determined by newly activated plastic events occurring during the relaxation process, a scenario consistent with the phenomenology of avalanche dynamics in the low shear rate limit of steadily sheared amorphous solids. Our simplified coarse grained description not only allows capturing the phenomenology of residual stress states but also rationalising the altered material properties that are probed using small and large deformation protocols applied to the relaxed material.
在软非晶材料中,大剪切变形后的剪切停止会导致材料具有残余剪应力的构型。尽管这些状态的起源以及材料内部局部剪应力的分布对于材料性能的变化及其后续应用很重要,但目前尚未得到很好的理解。在这项工作中,我们使用一种模型致密非布朗软非晶材料的分子动力学模拟来探究向残余应力状态的非平凡弛豫过程。我们发现,与热玻璃类似,在剪切停止之前剪切速率的增加会导致残余应力状态降低。我们使用一种细观弹塑性描述来解释我们的发现,该描述明确包括对局部剪切转变的长程弹性响应。我们发现,在流动停止后,初始应力弛豫确实取决于预剪切应力状态,但最终残余应力主要由弛豫过程中发生的新激活的塑性事件决定,这种情况与在稳定剪切非晶固体的低剪切速率极限下的雪崩动力学现象一致。我们简化的粗粒化描述不仅能够捕捉残余应力状态的现象学,还能解释使用应用于弛豫材料的小变形和大变形协议所探测到的材料性能变化。