Department of Atmospheric Science, University of Wyoming , 1000 East University Avenue, Laramie, Wyoming 82071, United States.
All4, Inc. , Kimberton, Pennsylvania 19442, United States.
Environ Sci Technol. 2017 Aug 1;51(15):8832-8840. doi: 10.1021/acs.est.7b00571. Epub 2017 Jul 12.
Atmospheric methane emissions from active natural gas production sites in normal operation were quantified using an inverse Gaussian method (EPA's OTM 33a) in four major U.S. basins/plays: Upper Green River (UGR, Wyoming), Denver-Julesburg (DJ, Colorado), Uintah (Utah), and Fayetteville (FV, Arkansas). In DJ, Uintah, and FV, 72-83% of total measured emissions were from 20% of the well pads, while in UGR the highest 20% of emitting well pads only contributed 54% of total emissions. The total mass of methane emitted as a percent of gross methane produced, termed throughput-normalized methane average (TNMA) and determined by bootstrapping measurements from each basin, varied widely between basins and was (95% CI): 0.09% (0.05-0.15%) in FV, 0.18% (0.12-0.29%) in UGR, 2.1% (1.1-3.9%) in DJ, and 2.8% (1.0-8.6%) in Uintah. Overall, wet-gas basins (UGR, DJ, Uintah) had higher TNMA emissions than the dry-gas FV at all ranges of production per well pad. Among wet basins, TNMA emissions had a strong negative correlation with average gas production per well pad, suggesting that consolidation of operations onto single pads may reduce normalized emissions (average number of wells per pad is 5.3 in UGR versus 1.3 in Uintah and 2.8 in DJ).
采用反向高斯法(EPA 的 OTM 33a),在美国四个主要的天然气产区/盆地(怀俄明州上绿河、科罗拉多州丹佛-朱尔斯堡、犹他州尤因塔和阿肯色州费耶特维尔)对正常运行的活跃天然气生产站点的大气甲烷排放进行了量化。在 DJ、Uintah 和 FV,20%的井场贡献了总排放量的 72-83%,而在 UGR,排放最高的 20%的井场仅贡献了总排放量的 54%。作为总甲烷排放量与总甲烷产量的百分比,即通过从每个盆地的测量数据进行自举法确定的甲烷平均吞吐量归一化(TNMA),在盆地之间差异很大,范围为:FV(95%置信区间)为 0.09%(0.05-0.15%),UGR 为 0.18%(0.12-0.29%),DJ 为 2.1%(1.1-3.9%),Uintah 为 2.8%(1.0-8.6%)。总体而言,湿天然气盆地(UGR、DJ、Uintah)的 TNMA 排放量在每个井场的产量范围内均高于干气盆地 FV。在湿天然气盆地中,TNMA 排放量与每口井的平均天然气产量呈强烈负相关,这表明将运营整合到单个井场可能会减少归一化排放量(UGR 中每井场的平均井数为 5.3,而 Uintah 和 DJ 分别为 1.3 和 2.8)。