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金属纳米结构中表面等离子体共振的塑造：非线性介电常数对系统尺寸和温度的依赖性。

Molding of Plasmonic Resonances in Metallic Nanostructures: Dependence of the Non-Linear Electric Permittivity on System Size and Temperature.

作者信息

Alabastri Alessandro, Tuccio Salvatore, Giugni Andrea, Toma Andrea, Liberale Carlo, Das Gobind, Angelis Francesco De, Fabrizio Enzo Di, Zaccaria Remo Proietti

机构信息

Istituto Italiano di Tecnologia, Via Morego 30, Genova 16163, Italy.

King Abdullah University of Science and Technology (KAUST), Physical Science and Engineering (PSE) Division, Biological and Environmental Science and Engineering (BESE) Division, Thuwal 23955-6900, Kingdom of Saudi Arabia.

出版信息

Materials (Basel). 2013 Oct 25;6(11):4879-4910. doi: 10.3390/ma6114879.

DOI:10.3390/ma6114879
PMID:28788366
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5452772/
Abstract

In this paper, we review the principal theoretical models through which the dielectric function of metals can be described. Starting from the Drude assumptions for intraband transitions, we show how this model can be improved by including interband absorption and temperature effect in the damping coefficients. Electronic scattering processes are described and included in the dielectric function, showing their role in determining plasmon lifetime at resonance. Relationships among permittivity, electric conductivity and refractive index are examined. Finally, a temperature dependent permittivity model is presented and is employed to predict temperature and non-linear field intensity dependence on commonly used plasmonic geometries, such as nanospheres.

摘要

在本文中，我们回顾了用于描述金属介电函数的主要理论模型。从带内跃迁的德鲁德假设出发，我们展示了如何通过在阻尼系数中纳入带间吸收和温度效应来改进该模型。描述了电子散射过程并将其纳入介电函数，展示了它们在确定共振时等离子体激元寿命中的作用。研究了介电常数、电导率和折射率之间的关系。最后，提出了一个与温度相关的介电常数模型，并将其用于预测温度以及常用等离子体几何结构（如纳米球）对非线性场强的依赖性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/558e/5452772/a7ea0124102f/materials-06-04879-g016.jpg
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