Sakumichi Naoyuki, Okumura Ko
Soft Matter Center, Ochanomizu University, Bunkyo-ku, Tokyo, 112-8610, Japan.
Department of Physics, Ochanomizu University, Bunkyo-ku, Tokyo, 112-8610, Japan.
Sci Rep. 2017 Aug 14;7(1):8065. doi: 10.1038/s41598-017-07214-8.
Needs to impart appropriate elasticity and high toughness to viscoelastic polymer materials are ubiquitous in industries such as concerning automobiles and medical devices. One of the major problems to overcome for toughening is catastrophic failure linked to a velocity jump, i.e., a sharp transition in the velocity of crack propagation occurred in a narrow range of the applied load. However, its physical origin has remained an enigma despite previous studies over 60 years. Here, we propose an exactly solvable model that exhibits the velocity jump incorporating linear viscoelasticity with a cutoff length for a continuum description. With the exact solution, we elucidate the physical origin of the velocity jump: it emerges from a dynamic glass transition in the vicinity of the propagating crack tip. We further quantify the velocity jump together with slow- and fast-velocity regimes of crack propagation, which would stimulate the development of tough polymer materials.
在汽车和医疗设备等行业中,赋予粘弹性聚合物材料适当弹性和高韧性的需求无处不在。增韧需要克服的主要问题之一是与速度跃升相关的灾难性失效,即在窄范围的外加载荷下裂纹扩展速度发生急剧转变。然而,尽管此前已有60多年的研究,但这种现象的物理根源仍是个谜。在此,我们提出一个精确可解的模型,该模型通过结合线性粘弹性和截止长度来描述连续介质,从而展现出速度跃升现象。借助精确解,我们阐明了速度跃升的物理根源:它源于裂纹扩展尖端附近的动态玻璃化转变。我们还进一步量化了速度跃升以及裂纹扩展的慢速和快速速度区域,这将推动坚韧聚合物材料的发展。