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青藏高原冰川雪坑中左旋葡聚糖和溶解有机碳的含量及其空间分布。

Levels and spatial distributions of levoglucosan and dissolved organic carbon in snowpits over the Tibetan Plateau glaciers.

机构信息

State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, CAS, Lanzhou 730000, China.

Shanxi Key Laboratory of Earth Surface System and Environmental Carrying Capacity, Xi'an, 710127, China; Institute of Earth Surface System and Hazards, Northwest University, Xi'an 710127, China; College of Urban and Environmental Sciences, Northwest University, Xi'an 710127, China.

出版信息

Sci Total Environ. 2018 Jan 15;612:1340-1347. doi: 10.1016/j.scitotenv.2017.08.267. Epub 2017 Sep 25.

Abstract

In this study, we collected 60 snowpit samples in nine glaciers from the northern to the southern Tibetan Plateau (TP), to study the levels and spatial distributions of levoglucosan and dissolved organic carbon (DOC). The lowest concentration of levoglucosan was found in the Yuzhufeng (YZF) glacier with a mean value of 0.24±0.08ngmL, while the highest concentration of levoglucosan was detected in the Gurenhekou (GRHK) glacier with a mean value of 11.72±15.61ngmL. However, the average DOC concentration in TP glaciers were comparable, without significant regional differences. The levoglucosan/DOC ratio ranged from 0.02 to 6.03% in the Tibetan Plateau glaciers. This ratios and the correlations between levoglucosan and DOC suggested that biomass burning products contributed only marginally to DOC levels in the TP glaciers. Moreover, the analysis of air mass backward trajectories suggested that levoglucosan and DOC in TP glaciers should be transported from the northwestern TP, internal TP, Central Asia, South and East Asia regions.

摘要

在这项研究中,我们在青藏高原(TP)从北到南的 9 条冰川中收集了 60 个雪坑样本,以研究左旋葡聚糖和溶解有机碳(DOC)的水平和空间分布。左旋葡聚糖浓度最低的是玉珠峰(YZF)冰川,平均值为 0.24±0.08ngmL,而左旋葡聚糖浓度最高的是古里雅口(GRHK)冰川,平均值为 11.72±15.61ngmL。然而,TP 冰川的平均 DOC 浓度相当,没有明显的区域差异。青藏高原冰川的左旋葡聚糖/DOC 比值范围为 0.02 至 6.03%。这些比值以及左旋葡聚糖和 DOC 之间的相关性表明,生物量燃烧产物对 TP 冰川的 DOC 水平的贡献微不足道。此外,气团后向轨迹分析表明,TP 冰川中的左旋葡聚糖和 DOC 应该是从青藏高原西北部、内部、中亚、南亚和东亚地区输送而来的。

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