Chen Zhi-Guo, Wang Luyang, Song Yu, Lu Xingye, Luo Huiqian, Zhang Chenglin, Dai Pengcheng, Yin Zhiping, Haule Kristjan, Kotliar Gabriel
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Institute for Advanced Study, Tsinghua University, Beijing 100084, China.
Phys Rev Lett. 2017 Sep 1;119(9):096401. doi: 10.1103/PhysRevLett.119.096401. Epub 2017 Aug 31.
We report infrared studies of AFe_{2}As_{2} (A=Ba, Sr), two representative parent compounds of iron-arsenide superconductors, at magnetic fields (B) up to 17.5 T. Optical transitions between Landau levels (LLs) were observed in the antiferromagnetic states of these two parent compounds. Our observation of a sqrt[B] dependence of the LL transition energies, the zero-energy intercepts at B=0 T under the linear extrapolations of the transition energies and the energy ratio (∼2.4) between the observed LL transitions, combined with the linear band dispersions in two-dimensional (2D) momentum space obtained by theoretical calculations, demonstrates the existence of massless Dirac fermions in the antiferromagnet BaFe_{2}As_{2}. More importantly, the observed dominance of the zeroth-LL-related absorption features and the calculated bands with extremely weak dispersions along the momentum direction k_{z} indicate that massless Dirac fermions in BaFe_{2}As_{2} are 2D. Furthermore, we find that the total substitution of the barium atoms in BaFe_{2}As_{2} by strontium atoms not only maintains 2D massless Dirac fermions in this system, but also enhances their Fermi velocity, which supports that the Dirac points in iron-arsenide parent compounds are topologically protected.
我们报道了对铁砷化物超导体的两种代表性母体化合物AFe₂As₂(A = Ba,Sr)在高达17.5 T的磁场(B)下的红外研究。在这两种母体化合物的反铁磁状态中观察到了朗道能级(LLs)之间的光学跃迁。我们观察到LL跃迁能量对√B的依赖性、在跃迁能量线性外推下B = 0 T时的零能量截距以及观察到的LL跃迁之间的能量比(约为2.4),再结合理论计算得到的二维(2D)动量空间中的线性能带色散,证明了反铁磁体BaFe₂As₂中无质量狄拉克费米子的存在。更重要的是,观察到的与零级LL相关的吸收特征的主导地位以及计算得到的沿动量方向kz色散极弱的能带表明,BaFe₂As₂中的无质量狄拉克费米子是二维的。此外,我们发现用锶原子完全取代BaFe₂As₂中的钡原子不仅能在该系统中保持二维无质量狄拉克费米子,还能提高它们的费米速度,这支持了铁砷化物母体化合物中的狄拉克点是拓扑保护的。