College of Environment, Research Center of Environmental Science, Key Laboratory of Microbial Technology for Industrial Pollution Control of Zhejiang Province, Zhejiang University of Technology, Hangzhou, 310014, China.
Zhejiang Province Environmental Monitoring Center, Hangzhou, 310012, China.
Environ Sci Pollut Res Int. 2017 Dec;24(35):27436-27444. doi: 10.1007/s11356-017-0339-x. Epub 2017 Oct 4.
Troposphere ozone, which is from secondary formation processes, has been increasing dramatically during the last decades in China, inducing high health risks. In this study, temporal and spatial distribution of O was studied among 13 sites of three cities during 2014-2016. The objectives were to clarify the characteristics of the ambient pollution of O under the influence from other pollutants and meteorological parameters and the health outcomes from exposure to O. The concentrations of O during summer were much higher than those during winter, and the concentrations in downtown areas were higher than in rural or mountain areas. PM, NO, SO, and wind speed (WS) were negatively correlated with O, and CO, temperature (T), and relative humidity (RH) were positively correlated with O. In multivariable analysis, two separate factors-solar radiation and atmospheric diffusion status, affected the O levels. The concentrations of O reached the highest level at 15:00 and the lowest value at about 6:00-8:00, with the similar trend to T and WS, and opposite to RH. According to the dose-response model, relative risks (RRs) and population attributable fractions (PAFs) with confidence intervals (CIs) for chronic obstructive pulmonary disease (COPD) from exposure to O were 1.0612 (CI 1.0607-1.0616) and 5.32% (CI 5.29-5.36%), respectively, attributable to 2000 deaths in Zhejiang Province in 2014.
对流层臭氧主要来源于二次形成过程,过去几十年来,中国的对流层臭氧浓度急剧增加,导致健康风险上升。本研究于 2014-2016 年在三个城市的 13 个点位,研究了臭氧的时空分布,目的是阐明在其他污染物和气象参数的影响下,臭氧环境污染物的特征以及暴露于臭氧产生的健康后果。夏季臭氧浓度明显高于冬季,城区臭氧浓度高于农村或山区。臭氧与 PM、NO、SO 和风速(WS)呈负相关,与 CO、温度(T)和相对湿度(RH)呈正相关。多变量分析表明,两个单独的因素——太阳辐射和大气扩散状况,影响了臭氧水平。臭氧浓度在 15 时达到最高水平,约在 6 时-8 时达到最低水平,其变化趋势与 T 和 WS 相似,与 RH 相反。根据剂量反应模型,COPD 暴露的相对风险(RR)和人群归因分数(PAF)及其置信区间(CI)分别为 1.0612(CI 1.0607-1.0616)和 5.32%(CI 5.29-5.36%),归因于 2014 年浙江省 2000 例 COPD 死亡。