Lahneman D J, Huffman T J, Xu Peng, Wang S L, Grogan T, Qazilbash M M
Opt Express. 2017 Aug 21;25(17):20421-20430. doi: 10.1364/OE.25.020421.
Scattering-type scanning near-field optical microscopy (S-SNOM) has enormous potential as a spectroscopy tool in the infrared spectral range where it can probe phonon resonances and carrier dynamics at the nanometer lengths scales. However, its applicability is limited by the lack of practical and affordable table-top light sources emitting intense broadband infrared radiation in the 100 cm to 2,500 cm spectral range. This paper introduces a high temperature plasma light source that is both ultra-broadband and has much more radiant power in the infrared spectral range than conventional, table-top thermal light sources such as the globar. We implement this plasma lamp in our near-field optical spectroscopy set up and demonstrate its capability as a broadband infrared nano-spectroscopy light source by obtaining near-field infrared amplitude and phase spectra of the phonon resonances of SiO and SrTiO.
散射型扫描近场光学显微镜(S-SNOM)作为一种光谱工具,在红外光谱范围内具有巨大潜力,它能够在纳米尺度上探测声子共振和载流子动力学。然而,其应用受到限制,因为缺乏实用且价格合理的桌面光源,无法在100厘米至2500厘米的光谱范围内发射高强度宽带红外辐射。本文介绍了一种高温等离子体光源,它不仅超宽带,而且在红外光谱范围内比传统的桌面热光源(如碳硅棒)具有更高的辐射功率。我们在近场光学光谱装置中使用了这种等离子体灯,并通过获取SiO和SrTiO声子共振的近场红外振幅和相位光谱,展示了其作为宽带红外纳米光谱光源的能力。